Progress and challenges of metal-organic frameworks-based materials for SR-AOPs applications in water treatment

被引：182

作者：

Huang, Danlian ^{[1
,2
]}

Zhang, Gaoxia ^{[1
,2
]}

Yi, Jing ^{[1
,2
]}

Cheng, Min ^{[1
,2
]}

Lai, Cui ^{[1
,2
]}

Xu, Piao ^{[1
,2
]}

Zhang, Chen ^{[1
,2
]}

Liu, Yang ^{[1
,2
]}

Zhou, Chengyun ^{[1
,2
]}

Xue, Wenjing ^{[1
,2
]}

Wang, Rongzhong ^{[1
,2
]}

Li, Zhihao ^{[1
,2
]}

Chen, Sha ^{[1
,2
]}

机构：

[1] Hunan Univ, Coll Environm Sci & Engn, Changsha 410082, Hunan, Peoples R China

[2] Hunan Univ, Minist Educ, Key Lab Environm Biol & Pollut Control, Changsha 410082, Hunan, Peoples R China

来源：

CHEMOSPHERE | 2021年 / 263卷

基金：

中国国家自然科学基金;

关键词：

Metal-organic frameworks; Sulfate radical based advanced oxidation processes; Organic pollutant degradation; Catalytic mechanism; ACID ORANGE 7; HETEROGENEOUS PERSULFATE CATALYST; WALLED CARBON NANOTUBES; PHOTO-FENTON CATALYST; BISPHENOL-A; PHOTOCATALYTIC DEGRADATION; ADVANCED OXIDATION; RHODAMINE-B; WASTE-WATER; PEROXYMONOSULFATE ACTIVATION;

D O I：

10.1016/j.chemosphere.2020.127672

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

As environmental problems become more and more severe, sulfate radical (SO4 center dot-) based advanced oxidation processes (SR-AOPs) are widely recognized for their high removal efficiency of recalcitrant organic pollutants in water. Metal-organic frameworks (MOFs) have attracted wide attention in SR-AOPs due to their outstanding properties (e.g. large surface area, ultra-high porosity, and diversity of material design, etc). Herein, we present an overview of the development and challenges in the synthesis of different types of MOFs, combination of MOFs with other materials (metal centers, conductors, cellulose, etc.) and the construction of catalysts with special structures (core-shell structures and hollow structures) as well as their applications in SR-AOPs for the degradation of organic pollutants. Several review papers have already mentioned the application of a branch of MOFs or simple composites of MOFs in SR-AOP, whereas the latest progresses on the application of MOFs-based materials to SR-AOPs was described rarely. Besides, the degradation mechanism of MOFs as catalysts has not been systematically discussed. To this end, the mechanisms of MOFs and MOF-based materials as catalysts to activate PMS/PS in different systems are analyzed, including radicals and non-radicals pathways. Meanwhile, considering that the research in this field is still in its infancy, a lot of improvements are still needed to effectively promote and implement this technology. (C) 2020 Elsevier Ltd. All rights reserved.

引用

页数：25

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