Assembly of porous lanthanide metal-organic frameworks constructed by chalcone dicarboxylic acid and exploration of their properties

被引：20

作者：

Pan, Wei ^{[1
,2
,4
]}

Gong, Chunhua ^{[2
,4
]}

Zeng, Xianghua ^{[2
,4
]}

Hu, Chenyan ^{[2
]}

Zhang, Yi ^{[2
]}

Zhu, Dun-Ru ^{[1
]}

Xu, Hao ^{[2
]}

Guo, Haiyang ^{[2
]}

Zhang, Junyong ^{[2
,4
]}

Xie, Jingli ^{[2
,3
,4
]}

机构：

[1] Nanjing Tech Univ, Coll Chem Engn, Nanjing 211816, Jiangsu, Peoples R China

[2] Jiaxing Univ, Coll Biol Chem Sci & Engn, Jiaxing 314001, Peoples R China

[3] GTIIT, Guangdong Prov Lab Chem & Fine Chem Engn Shantou, 241 Daxue Rd, Shantou 515063, Guangdong, Peoples R China

[4] Chinese Acad Sci, Fujian Inst Res Struct Matter, State Key Lab Struct Chem, Fuzhou 350002, Fujian, Peoples R China

来源：

POLYHEDRON | 2019年 / 169卷

基金：

中国国家自然科学基金;

关键词：

Metal-organic frameworks; Lanthanide; Solvothermal; Porosity; Dye degradation; COORDINATION POLYMERS; LN-MOF; LUMINESCENT; PHOTOLUMINESCENCE; DEGRADATION; CATALYSTS; REMOVAL; SENSOR;

D O I：

10.1016/j.poly.2019.04.062

中图分类号：

O61 [无机化学];

学科分类号：

070301 ; 081704 ;

摘要：

Using rational designed chalcone dicarboxylic acid ligand (H2L), a series of lanthanide metal-organic frameworks (Ln-MOFs) with the general formula Ln(HL)(3) (Ln = La; Ce; Pr; Nd; Sm; Eu; Gd) have been obtained under the solvothermal reaction. The crystal structure analysis displays that all the Ln-MOFs are the isomorphic three-dimensional (3D) metal-organic frameworks with honeycomb cavities, in which the porosity is similar to 20% that calculated via PLATON software. In addition, photocatalytic activities of Ln-MOFs for the degradation of several organic dyes have been explored, suggesting that Ln-MOFs can be used as efficient heterogeneous photocatalyst for the degradation of organic dyes. (C) 2019 Elsevier Ltd. All rights reserved.

引用

页码：24 / 31

页数：8

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