A perspective on high-entropy two-dimensional materials

被引:45
作者
Cui, Yanglansen [1 ]
Zhang, Yongzheng [1 ]
Cao, Zhenjiang [1 ]
Gu, Jianan [1 ]
Du, Zhiguo [1 ]
Li, Bin [1 ]
Yang, Shubin [1 ]
机构
[1] Beihang Univ, Sch Mat Sci & Engn, Beijing 100191, Peoples R China
来源
SUSMAT | 2022年 / 2卷 / 01期
基金
中国博士后科学基金; 北京市自然科学基金; 中国国家自然科学基金;
关键词
2D materials; high-entropy; lattice distortions; MXenes; strong stress; VAN; CONVERSION; PHASE;
D O I
10.1002/sus2.47
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
In past decades, high-entropy (HE) materials, containing five or more elements with approximately equal atomic ratio, are extensively investigated due to their desirable properties in a series of applications. Recently, HE two-dimensional (2D) materials have become promising materials, which not only endow the advantages from their bulk form but also exhibit unusual properties due to their 2D features. So far, the HE 2D transition metal carbides (MXenes), dichalcogenides (TMDs), hydrotalcites (LDHs), and oxides have been successfully synthesized and performed well in different electrochemical reactions, which is originated from the synergistic effect of multicomponents and atomic thin characteristics. Here, the challenges on processing, characterization, and property predictions of HE 2D materials are emphasized. Finally, viable strategies, advanced processing, fundamental understanding, in-depth characterization of new HE 2D materials are proposed.
引用
收藏
页码:65 / 75
页数:11
相关论文
共 51 条
[1]   Functionalizing MXenes by Tailoring Surface Terminations in Different Chemical Environments [J].
Bjork, Jonas ;
Rosen, Johanna .
CHEMISTRY OF MATERIALS, 2021, 33 (23) :9108-9118
[2]   2D High-Entropy Transition Metal Dichalcogenides for Carbon Dioxide Electrocatalysis [J].
Cavin, John ;
Ahmadiparidari, Alireza ;
Majidi, Leily ;
Thind, Arashdeep Singh ;
Misal, Saurabh N. ;
Prajapati, Aditya ;
Hemmat, Zahra ;
Rastegar, Sina ;
Beukelman, Andrew ;
Singh, Meenesh R. ;
Unocic, Kinga A. ;
Salehi-Khojin, Amin ;
Mishra, Rohan .
ADVANCED MATERIALS, 2021, 33 (31)
[3]   Metal-Guided Selective Growth of 2D Materials: Demonstration of a Bottom-Up CMOS Inverter [J].
Chiu, Ming-Hui ;
Tang, Hao-Ling ;
Tseng, Chien-Chih ;
Han, Yimo ;
Aljarb, Areej ;
Huang, Jing-Kai ;
Wan, Yi ;
Fu, Jui-Han ;
Zhang, Xixiang ;
Chang, Wen-Hao ;
Muller, David A. ;
Takenobu, Taishi ;
Tung, Vincent ;
Li, Lain-Jong .
ADVANCED MATERIALS, 2019, 31 (18)
[4]   High-Entropy Metal Sulfide Nanoparticles Promise High-Performance Oxygen Evolution Reaction [J].
Cui, Mingjin ;
Yang, Chunpeng ;
Li, Boyang ;
Dong, Qi ;
Wu, Meiling ;
Hwang, Sooyeon ;
Xie, Hua ;
Wang, Xizheng ;
Wang, Guofeng ;
Hu, Liangbing .
ADVANCED ENERGY MATERIALS, 2021, 11 (03)
[5]   Tungsten Oxide/Carbide Surface Heterojunction Catalyst with High Hydrogen Evolution Activity [J].
Cui, Yanglansen ;
Tan, Xin ;
Xiao, Kefeng ;
Zhao, Shenlong ;
Bedford, Nicholas M. ;
Liu, Yuefeng ;
Wang, Zichun ;
Wu, Kuang-Hsu ;
Pan, Jian ;
Saputera, Wibawa Hendra ;
Cheong, Soshan ;
Tilley, Richard D. ;
Smith, Sean C. ;
Yun, Jimmy ;
Dai, Liming ;
Amal, Rose ;
Wang, Da-Wei .
ACS ENERGY LETTERS, 2020, 5 (11) :3560-3568
[6]   Refilling Nitrogen to Oxygen Vacancies in Ultrafine Tungsten Oxide Clusters for Superior Lithium Storage [J].
Cui, Yanglansen ;
Xiao, Kefeng ;
Bedford, Nicholas M. ;
Lu, Xinxin ;
Yun, Jimmy ;
Amal, Rose ;
Wang, Da-Wei .
ADVANCED ENERGY MATERIALS, 2019, 9 (37)
[7]   Bulk high-entropy nitrides and carbonitrides [J].
Dippo, Olivia F. ;
Mesgarzadeh, Neda ;
Harrington, Tyler J. ;
Schrader, Grant D. ;
Vecchio, Kenneth S. .
SCIENTIFIC REPORTS, 2020, 10 (01)
[8]   Unlocking the catalytic activities of 2H-phase Mo-based compounds via topological conversion reaction [J].
Du, Zhiguo ;
Wang, Shuai ;
Hu, Riming ;
Zhang, Di ;
Gu, Jianan ;
Chen, Xiao ;
Shang, Jiaxiang ;
Li, Bin ;
Yang, Shubin ;
Guo, Lin .
MATERIALS TODAY, 2021, 51 :136-144
[9]   High-Entropy Carbonitride MAX Phases and Their Derivative MXenes [J].
Du, Zhiguo ;
Wu, Cheng ;
Chen, Yuchuan ;
Zhu, Qi ;
Cui, Yanglansen ;
Wang, Haiyang ;
Zhang, Yongzheng ;
Chen, Xiao ;
Shang, Jiaxiang ;
Li, Bin ;
Chen, Weihua ;
Liu, Chuntai ;
Yang, Shubin .
ADVANCED ENERGY MATERIALS, 2022, 12 (06)
[10]   High-Throughput Production of 1T MoS2 Monolayers Based on Controllable Conversion of Mo-Based MXenes [J].
Du, Zhiguo ;
Guo, Yu ;
Wang, Haiyang ;
Gu, Jianan ;
Zhang, Yongzheng ;
Cheng, Zongju ;
Li, Bin ;
Li, Songmei ;
Yang, Shubin .
ACS NANO, 2021, 15 (12) :19275-19283