Excitation wavelength independent visible color emission of carbon dots

被引:416
作者
Wang, Hua [1 ,2 ]
Sun, Chun [1 ]
Chen, Xingru [1 ,3 ]
Zhang, Yu [1 ]
Colvin, Vicki L. [4 ]
Rice, Quinton [5 ]
Seo, Jaetae [5 ]
Feng, Shengyu [6 ]
Wang, Shengnian [2 ]
Yu, William W. [1 ,3 ]
机构
[1] Jilin Univ, Coll Elect Sci & Engn, State Key Lab Integrated Optoelect, Changchun 130012, Peoples R China
[2] Louisiana Tech Univ, Dept Chem Engn, Inst Micromfg, Ruston, LA 71270 USA
[3] Louisiana State Univ, Dept Chem & Phys, Shreveport, LA 71115 USA
[4] Brown Univ, Dept Chem, Providence, RI 02912 USA
[5] Hampton Univ, Dept Phys, Adv Ctr Laser Sci & Spect, Hampton, VA 23668 USA
[6] Shandong Univ, Sch Chem & Chem Engn, Jinan 250100, Peoples R China
基金
美国国家科学基金会;
关键词
QUANTUM DOTS; FLUORESCENT; PHOTOLUMINESCENCE; STATE; LUMINESCENCE; THICKNESS; MICELLES; NANODOTS; GREEN;
D O I
10.1039/c6nr09200d
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Carbon dots (CDs) usually emit a strong blue light and excitation wavelength dependent long wavelength lights. This significantly limits their applications because one has to use a series of different excitation light sources to get different colors and the long wavelength emissions are usually very weak. We found that one type of CDs synthesized from p-phenylenediamine could emit various long wavelength lights (green to red) independent of the excitation wavelength when dispersed in different solvents. The photoluminescence quantum yields of the same CDs were 10-35% in different solvents for different color emissions. Based on this solvent-color effect, we further mixed the same CDs with different polymers to form solid CD films for various color emissions, and these film emissions were also excitation wavelength independent. Multicolor LEDs were demonstrated with the same CDs in solution and solid film states for color displays.
引用
收藏
页码:1909 / 1915
页数:7
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