Discovery of a New Intermediate Enables One-Step Deposition of High-Quality Perovskite Films via Solvent Engineering
被引:28
|
作者:
Hu, Chen
论文数: 0引用数: 0
h-index: 0
机构:
Hong Kong Univ Sci & Technol, Dept Chem, Kowloon, Clear Water Bay, Hong Kong, Peoples R ChinaHong Kong Univ Sci & Technol, Dept Chem, Kowloon, Clear Water Bay, Hong Kong, Peoples R China
Hu, Chen
[1
]
Shivarudraiah, Sunil B.
论文数: 0引用数: 0
h-index: 0
机构:
Hong Kong Univ Sci & Technol, Dept Chem, Kowloon, Clear Water Bay, Hong Kong, Peoples R ChinaHong Kong Univ Sci & Technol, Dept Chem, Kowloon, Clear Water Bay, Hong Kong, Peoples R China
Shivarudraiah, Sunil B.
[1
]
Sung, Herman H. Y.
论文数: 0引用数: 0
h-index: 0
机构:
Hong Kong Univ Sci & Technol, Dept Chem, Kowloon, Clear Water Bay, Hong Kong, Peoples R ChinaHong Kong Univ Sci & Technol, Dept Chem, Kowloon, Clear Water Bay, Hong Kong, Peoples R China
Sung, Herman H. Y.
[1
]
Williams, Ian D.
论文数: 0引用数: 0
h-index: 0
机构:
Hong Kong Univ Sci & Technol, Dept Chem, Kowloon, Clear Water Bay, Hong Kong, Peoples R ChinaHong Kong Univ Sci & Technol, Dept Chem, Kowloon, Clear Water Bay, Hong Kong, Peoples R China
Williams, Ian D.
[1
]
Halpert, Jonathan E.
论文数: 0引用数: 0
h-index: 0
机构:
Hong Kong Univ Sci & Technol, Dept Chem, Kowloon, Clear Water Bay, Hong Kong, Peoples R ChinaHong Kong Univ Sci & Technol, Dept Chem, Kowloon, Clear Water Bay, Hong Kong, Peoples R China
Halpert, Jonathan E.
[1
]
Yang, Shihe
论文数: 0引用数: 0
h-index: 0
机构:
Hong Kong Univ Sci & Technol, Dept Chem, Kowloon, Clear Water Bay, Hong Kong, Peoples R China
Peking Univ, Shenzhen Grad Sch, Sch Chem Biol & Biotechnol, Guangdong Prov Key Lab Nanomicro Mat Res, Shenzhen 518055, Peoples R ChinaHong Kong Univ Sci & Technol, Dept Chem, Kowloon, Clear Water Bay, Hong Kong, Peoples R China
Yang, Shihe
[1
,2
]
机构:
[1] Hong Kong Univ Sci & Technol, Dept Chem, Kowloon, Clear Water Bay, Hong Kong, Peoples R China
[2] Peking Univ, Shenzhen Grad Sch, Sch Chem Biol & Biotechnol, Guangdong Prov Key Lab Nanomicro Mat Res, Shenzhen 518055, Peoples R China
film formations;
intermediates;
perovskite solar cells;
SOLAR-CELLS;
EFFICIENT;
D O I:
10.1002/solr.202000712
中图分类号:
TE [石油、天然气工业];
TK [能源与动力工程];
学科分类号:
0807 ;
0820 ;
摘要:
Bromide-based organo-metal halide perovskites have shown great potential for use in tandem solar cells (SCs), light-emitting diodes (LEDs), and photodetectors. Herein, a new protocol using a one-step deposition method for producing formamidinium lead bromide (FAPbBr(3)) perovskites is reported, which features a solvent-engineered intermediate phase to achieve superior films. For the first time, a FABr-PbBr2-DMSO intermediate is identified and single crystals of the same intermediate compound are synthesized. A systematic investigation of phase evolution in the film formation process reveals that DMSO enables crystallization of the FABr-PbBr2-DMSO intermediate and thus modulates the crystallization process of FAPbBr(3) perovskite, achieving uniform, smooth films with Volmer-Weber morphology. To prevent hole leakage arising from the larger bandgap of FAPbBr(3) than FAPbI(3), an additional layer of Mg-doped ZnO nanoparticles is added. As a result, inverted SCs using these solvent engineered films achieve power conversion efficiencies (PCEs) of up to 9.06%, the highest reported efficiency for inverted FAPbBr(3) perovskite devices.
机构:
Univ Kebangsaan Malaysia, Solar Energy Res Inst, Bangi 43600, Selangor, MalaysiaUniv Kebangsaan Malaysia, Solar Energy Res Inst, Bangi 43600, Selangor, Malaysia
Noh, Mohamad Firdaus Mohamad
Arzaee, Nurul Affiqah
论文数: 0引用数: 0
h-index: 0
机构:
Univ Kebangsaan Malaysia, Solar Energy Res Inst, Bangi 43600, Selangor, MalaysiaUniv Kebangsaan Malaysia, Solar Energy Res Inst, Bangi 43600, Selangor, Malaysia
Arzaee, Nurul Affiqah
Mumthas, Inzamam Nawas Nawas
论文数: 0引用数: 0
h-index: 0
机构:
Univ Kebangsaan Malaysia, Solar Energy Res Inst, Bangi 43600, Selangor, MalaysiaUniv Kebangsaan Malaysia, Solar Energy Res Inst, Bangi 43600, Selangor, Malaysia
Mumthas, Inzamam Nawas Nawas
Aadenan, Amin
论文数: 0引用数: 0
h-index: 0
机构:
Univ Kebangsaan Malaysia, Solar Energy Res Inst, Bangi 43600, Selangor, Malaysia
Univ Teknol MARA, Fac Sci Appl, Kuala Pilah 72000, Negeri Sembilan, MalaysiaUniv Kebangsaan Malaysia, Solar Energy Res Inst, Bangi 43600, Selangor, Malaysia
Aadenan, Amin
Saifuddin, Farah Husna
论文数: 0引用数: 0
h-index: 0
机构:
Univ Kebangsaan Malaysia, Solar Energy Res Inst, Bangi 43600, Selangor, MalaysiaUniv Kebangsaan Malaysia, Solar Energy Res Inst, Bangi 43600, Selangor, Malaysia
Saifuddin, Farah Husna
Syakirin, Abu Dzar Al-Ghiffari
论文数: 0引用数: 0
h-index: 0
机构:
Univ Kebangsaan Malaysia, Solar Energy Res Inst, Bangi 43600, Selangor, MalaysiaUniv Kebangsaan Malaysia, Solar Energy Res Inst, Bangi 43600, Selangor, Malaysia
Syakirin, Abu Dzar Al-Ghiffari
Mutalib, Muhazri Abd
论文数: 0引用数: 0
h-index: 0
机构:
Univ Kebangsaan Malaysia, Solar Energy Res Inst, Bangi 43600, Selangor, MalaysiaUniv Kebangsaan Malaysia, Solar Energy Res Inst, Bangi 43600, Selangor, Malaysia
Mutalib, Muhazri Abd
Lokman, Muhammad Quisar
论文数: 0引用数: 0
h-index: 0
机构:
Univ Kebangsaan Malaysia, Solar Energy Res Inst, Bangi 43600, Selangor, MalaysiaUniv Kebangsaan Malaysia, Solar Energy Res Inst, Bangi 43600, Selangor, Malaysia
Lokman, Muhammad Quisar
Ibrahim, Mohd Adib
论文数: 0引用数: 0
h-index: 0
机构:
Univ Kebangsaan Malaysia, Solar Energy Res Inst, Bangi 43600, Selangor, MalaysiaUniv Kebangsaan Malaysia, Solar Energy Res Inst, Bangi 43600, Selangor, Malaysia
Ibrahim, Mohd Adib
Teridi, Mohd Asri Mat
论文数: 0引用数: 0
h-index: 0
机构:
Univ Kebangsaan Malaysia, Solar Energy Res Inst, Bangi 43600, Selangor, MalaysiaUniv Kebangsaan Malaysia, Solar Energy Res Inst, Bangi 43600, Selangor, Malaysia
机构:
North China Elect Power Univ, Beijing Key Lab Novel Thin Film Solar Cells, Beijing 102206, Peoples R ChinaNorth China Elect Power Univ, Beijing Key Lab Novel Thin Film Solar Cells, Beijing 102206, Peoples R China
Ren, Yingke
Duan, Bin
论文数: 0引用数: 0
h-index: 0
机构:
Chinese Acad Sci, Hefei Inst Phys Sci, Inst Appl Technol, Key Lab Novel Thin Film Solar Cells, Hefei 230031, Peoples R ChinaNorth China Elect Power Univ, Beijing Key Lab Novel Thin Film Solar Cells, Beijing 102206, Peoples R China
Duan, Bin
Xu, Yafeng
论文数: 0引用数: 0
h-index: 0
机构:
Chinese Acad Sci, Hefei Inst Phys Sci, Inst Appl Technol, Key Lab Novel Thin Film Solar Cells, Hefei 230031, Peoples R ChinaNorth China Elect Power Univ, Beijing Key Lab Novel Thin Film Solar Cells, Beijing 102206, Peoples R China
Xu, Yafeng
Huang, Yang
论文数: 0引用数: 0
h-index: 0
机构:
Chinese Acad Sci, Hefei Inst Phys Sci, Inst Appl Technol, Key Lab Novel Thin Film Solar Cells, Hefei 230031, Peoples R ChinaNorth China Elect Power Univ, Beijing Key Lab Novel Thin Film Solar Cells, Beijing 102206, Peoples R China
Huang, Yang
Li, Zhaoqian
论文数: 0引用数: 0
h-index: 0
机构:
Chinese Acad Sci, Hefei Inst Phys Sci, Inst Appl Technol, Key Lab Novel Thin Film Solar Cells, Hefei 230031, Peoples R ChinaNorth China Elect Power Univ, Beijing Key Lab Novel Thin Film Solar Cells, Beijing 102206, Peoples R China
Li, Zhaoqian
Hu, Linhua
论文数: 0引用数: 0
h-index: 0
机构:
Chinese Acad Sci, Hefei Inst Phys Sci, Inst Appl Technol, Key Lab Novel Thin Film Solar Cells, Hefei 230031, Peoples R ChinaNorth China Elect Power Univ, Beijing Key Lab Novel Thin Film Solar Cells, Beijing 102206, Peoples R China
Hu, Linhua
Hayat, Tasawar
论文数: 0引用数: 0
h-index: 0
机构:
King Abdulaziz Univ, Dept Math, NAAM Res Grp, Fac Sci, Jeddah 21589, Saudi ArabiaNorth China Elect Power Univ, Beijing Key Lab Novel Thin Film Solar Cells, Beijing 102206, Peoples R China
Hayat, Tasawar
Wang, Hongxia
论文数: 0引用数: 0
h-index: 0
机构:
Queensland Univ Technol, Sch Chem Phys & Mech Engn, Brisbane, Qld 4001, AustraliaNorth China Elect Power Univ, Beijing Key Lab Novel Thin Film Solar Cells, Beijing 102206, Peoples R China
Wang, Hongxia
Zhu, Jun
论文数: 0引用数: 0
h-index: 0
机构:
Chinese Acad Sci, Hefei Inst Phys Sci, Inst Appl Technol, Key Lab Novel Thin Film Solar Cells, Hefei 230031, Peoples R ChinaNorth China Elect Power Univ, Beijing Key Lab Novel Thin Film Solar Cells, Beijing 102206, Peoples R China
Zhu, Jun
Dai, Songyuan
论文数: 0引用数: 0
h-index: 0
机构:
North China Elect Power Univ, Beijing Key Lab Novel Thin Film Solar Cells, Beijing 102206, Peoples R China
Chinese Acad Sci, Hefei Inst Phys Sci, Inst Appl Technol, Key Lab Novel Thin Film Solar Cells, Hefei 230031, Peoples R China
King Abdulaziz Univ, Dept Math, NAAM Res Grp, Fac Sci, Jeddah 21589, Saudi ArabiaNorth China Elect Power Univ, Beijing Key Lab Novel Thin Film Solar Cells, Beijing 102206, Peoples R China
机构:
Daegu Gyeongbuk Inst Sci Technol DGIST, Div Energy Technol, Daegu 42988, South KoreaDaegu Gyeongbuk Inst Sci Technol DGIST, Div Energy Technol, Daegu 42988, South Korea
Choi, Yong Chan
Jung, Kang-Won
论文数: 0引用数: 0
h-index: 0
机构:
Daegu Gyeongbuk Inst Sci Technol DGIST, Div Energy Technol, Daegu 42988, South KoreaDaegu Gyeongbuk Inst Sci Technol DGIST, Div Energy Technol, Daegu 42988, South Korea
机构:
Jinan Univ, Coll Informat Sci & Technol, Inst New Energy Technol, Guangzhou 510632, Guangdong, Peoples R ChinaJinan Univ, Coll Informat Sci & Technol, Inst New Energy Technol, Guangzhou 510632, Guangdong, Peoples R China
Guo, Fei
He, Wenxin
论文数: 0引用数: 0
h-index: 0
机构:
Jinan Univ, Coll Informat Sci & Technol, Inst New Energy Technol, Guangzhou 510632, Guangdong, Peoples R ChinaJinan Univ, Coll Informat Sci & Technol, Inst New Energy Technol, Guangzhou 510632, Guangdong, Peoples R China
He, Wenxin
Qiu, Shudi
论文数: 0引用数: 0
h-index: 0
机构:
Jinan Univ, Coll Informat Sci & Technol, Inst New Energy Technol, Guangzhou 510632, Guangdong, Peoples R ChinaJinan Univ, Coll Informat Sci & Technol, Inst New Energy Technol, Guangzhou 510632, Guangdong, Peoples R China
Qiu, Shudi
Wang, Chuan
论文数: 0引用数: 0
h-index: 0
机构:
Zhengzhou Univ, Natl Engn Res Ctr Adv Polymer Proc Technol, Zhengzhou 450002, Henan, Peoples R ChinaJinan Univ, Coll Informat Sci & Technol, Inst New Energy Technol, Guangzhou 510632, Guangdong, Peoples R China
Wang, Chuan
Liu, Xianhu
论文数: 0引用数: 0
h-index: 0
机构:
Zhengzhou Univ, Natl Engn Res Ctr Adv Polymer Proc Technol, Zhengzhou 450002, Henan, Peoples R ChinaJinan Univ, Coll Informat Sci & Technol, Inst New Energy Technol, Guangzhou 510632, Guangdong, Peoples R China
Liu, Xianhu
Forberich, Karen
论文数: 0引用数: 0
h-index: 0
机构:
Friedrich Alexander Univ Erlangen Nurnberg, Inst Mat Elect & Energy Technol i MEET, Martensstr 7, D-91058 Erlangen, GermanyJinan Univ, Coll Informat Sci & Technol, Inst New Energy Technol, Guangzhou 510632, Guangdong, Peoples R China
Forberich, Karen
Brabec, Christoph J.
论文数: 0引用数: 0
h-index: 0
机构:
Friedrich Alexander Univ Erlangen Nurnberg, Inst Mat Elect & Energy Technol i MEET, Martensstr 7, D-91058 Erlangen, Germany
Forschungszentrum Julich, Helmholtz Inst Erlangen Nurnberg Renewable Energy, Immerwahrstr 2, D-91058 Erlangen, GermanyJinan Univ, Coll Informat Sci & Technol, Inst New Energy Technol, Guangzhou 510632, Guangdong, Peoples R China
Brabec, Christoph J.
Mai, Yaohua
论文数: 0引用数: 0
h-index: 0
机构:
Jinan Univ, Coll Informat Sci & Technol, Inst New Energy Technol, Guangzhou 510632, Guangdong, Peoples R ChinaJinan Univ, Coll Informat Sci & Technol, Inst New Energy Technol, Guangzhou 510632, Guangdong, Peoples R China