Flexible CdS and PbS nanoparticles sensitized TiO2 nanotube arrays lead to significantly enhanced photocatalytic performance

被引:15
作者
Hou, Junwei [1 ]
Yang, Ye [1 ]
Zhou, Jingyi [1 ]
Wang, Yafei [1 ]
Xu, Tengze [1 ]
Wang, Qingyao [2 ]
机构
[1] China Univ Petr Beijing Karamay, State Key Lab Heavy Oil Proc, Karamay 834000, Peoples R China
[2] Ludong Univ, Sch Chem & Mat Sci, Yantai 264025, Peoples R China
基金
中国国家自然科学基金;
关键词
TiO2; NTAs; Ti mesh; CdS; PbS; Photocatalytic hydrogen generation; HYDROGEN GENERATION; ASSISTED SYNTHESIS; DOPED TIO2; MESH; DEGRADATION; FABRICATION; EVOLUTION; SYSTEM;
D O I
10.1016/j.ceramint.2020.08.041
中图分类号
TQ174 [陶瓷工业]; TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
TiO2 nanotube arrays (TiO2 NTAs) were mainly synthesized by the anodization of Ti foils, and the Ti mesh anodization was little researched. TiO2 NTAs/Ti mesh showed remarkably high photocatalytic performance in pollutant treatment and photocurrent/hydrogen generation. In this paper, TiO2 NTAs were synthesized on flexible three dimensional Ti mesh surface, and CdS/PbS sensitizers covered TiO2 NTAs by the hydrothermal deposition. Especially, the S-CdS photocatalyst prepared by CdS sensitization showed strong photocurrent and photocatalytic pollutant removal capacity. RhB, MB dyes and Cr(VI) ions were effectively purified under solar irradiation, and samples also showed excellent visible light-driven photoelectric ability. Furthermore, the S-PbS photocatalyst prepared by PbS sensitization showed high photocatalytic water splitting performance. The functional material offers a flexible, low cost and high photocatalytic membrane for waste water treatment and photocurrent/hydrogen generation.
引用
收藏
页码:28785 / 28791
页数:7
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