Possible charge disproportionation and new type charge localization in θ-(BEDT-TTF)2CsZn(SCN)4

被引:43
作者
Nakamura, T [1 ]
Minagawa, W [1 ]
Kinami, R [1 ]
Takahashi, T [1 ]
机构
[1] Gakushuin Univ, Dept Phys, Toshima Ku, Tokyo 1718588, Japan
关键词
organic conductor; BEDT-TTF; H-1-NMR; EPR; magnetic susceptibility; charge localization; electronic correlation;
D O I
10.1143/JPSJ.69.504
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
H-1-NMR, EPR and static magnetic susceptibility measurements have been performed on an organic conductor, theta-(BEDT-TTF)(2)CsZn(SCN)(4). The H-1-NMR-T-1(-1) and tie spin susceptibility exhibit anomalous enhancements at low temperatures. Around 20 K. where the spill susceptibility shows a minimum, the principal axes of the EPR g-tensor changed their directions, keeping the principal values constant. It indicates a possible change of the electronic nature. The low-temperature electronic state is discussed.
引用
收藏
页码:504 / 509
页数:6
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