Quantum metrology with a single spin-3/2 defect in silicon carbide

被引:37
作者
Soykal, O. O. [1 ]
Reinecke, T. L. [1 ]
机构
[1] Naval Res Lab, Washington, DC 20375 USA
关键词
AMBIENT CONDITIONS; ROOM-TEMPERATURE; COHERENT CONTROL; DIAMOND SPINS; QUBITS; DONOR; FIELD;
D O I
10.1103/PhysRevB.95.081405
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We show that implementations for quantum sensing with exceptional sensitivity and spatial resolution can be made using spin-3/2 semiconductor defect states. We illustrate this using the silicon monovacancy deep center in hexagonal SiC based on our rigorous derivation of this defect's ground state and of its electronic and optical properties. For a single V-Si(-) defect, we obtain magnetic field sensitivities capable of detecting individual nuclear magnetic moments. We also show that its zero-field splitting has an exceptional strain and temperature sensitivity within the technologically desirable near-infrared window of biological systems. The concepts and sensing schemes developed here are applicable to other point defects with half spin multiplet (S >= 3/2) configurations.
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页数:5
相关论文
共 39 条
[1]   Temperature Dependence of the Nitrogen-Vacancy Magnetic Resonance in Diamond [J].
Acosta, V. M. ;
Bauch, E. ;
Ledbetter, M. P. ;
Waxman, A. ;
Bouchard, L-S. ;
Budker, D. .
PHYSICAL REVIEW LETTERS, 2010, 104 (07)
[2]  
Altmann S.L., 1994, Point-group theory tables
[3]   Nanoscale imaging magnetometry with diamond spins under ambient conditions [J].
Balasubramanian, Gopalakrishnan ;
Chan, I. Y. ;
Kolesov, Roman ;
Al-Hmoud, Mohannad ;
Tisler, Julia ;
Shin, Chang ;
Kim, Changdong ;
Wojcik, Aleksander ;
Hemmer, Philip R. ;
Krueger, Anke ;
Hanke, Tobias ;
Leitenstorfer, Alfred ;
Bratschitsch, Rudolf ;
Jelezko, Fedor ;
Wrachtrup, Joerg .
NATURE, 2008, 455 (7213) :648-U46
[4]   Silicon vacancy in SiC as a promising quantum system for single-defect and single-photon spectroscopy [J].
Baranov, Pavel G. ;
Bundakova, Anna P. ;
Soltamova, Alexandra A. ;
Orlinskii, Sergei B. ;
Borovykh, Igor V. ;
Zondervan, Rob ;
Verberk, Rogier ;
Schmidt, Jan .
PHYSICAL REVIEW B, 2011, 83 (12)
[5]   Heralded entanglement between solid-state qubits separated by three metres [J].
Bernien, H. ;
Hensen, B. ;
Pfaff, W. ;
Koolstra, G. ;
Blok, M. S. ;
Robledo, L. ;
Taminiau, T. H. ;
Markham, M. ;
Twitchen, D. J. ;
Childress, L. ;
Hanson, R. .
NATURE, 2013, 497 (7447) :86-90
[6]   Spin coherence and echo modulation of the silicon vacancy in 4H-SiC at room temperature [J].
Carter, S. G. ;
Soykal, Oe. O. ;
Dev, Pratibha ;
Economou, Sophia E. ;
Glaser, E. R. .
PHYSICAL REVIEW B, 2015, 92 (16)
[7]  
Christle DJ, 2015, NAT MATER, V14, P160, DOI [10.1038/NMAT4144, 10.1038/nmat4144]
[8]  
Dolde F, 2011, NAT PHYS, V7, P459, DOI [10.1038/NPHYS1969, 10.1038/nphys1969]
[9]   Optical Polarization of Nuclear Spins in Silicon Carbide [J].
Falk, Abram L. ;
Klimov, Paul V. ;
Ivady, Viktor ;
Szasz, Krisztian ;
Christle, David J. ;
Koehl, William F. ;
Gali, Adam ;
Awschalom, David D. .
PHYSICAL REVIEW LETTERS, 2015, 114 (24)
[10]   Polytype control of spin qubits in silicon carbide [J].
Falk, Abram L. ;
Buckley, Bob B. ;
Calusine, Greg ;
Koehl, William F. ;
Dobrovitski, Viatcheslav V. ;
Politi, Alberto ;
Zorman, Christian A. ;
Feng, Philip X. -L. ;
Awschalom, David D. .
NATURE COMMUNICATIONS, 2013, 4