Synthesis, characterization and ion-binding properties of BODIPY scaffolds bearing sulfur function

被引：6
|
作者：
Zhao, Chunchang [1 ]
Li, Xia
Zhang, Jinxin
机构：
[1] E China Univ Sci & Technol, Key Lab Adv Mat, Shanghai 200237, Peoples R China
来源：
INORGANICA CHIMICA ACTA | 2014年 / 412卷
基金：
美国国家科学基金会;
关键词：
Borondipyrromethene-based probe; Synergic manner; Sulfur function; Oxidation state; SELECTIVE FLUORESCENT SENSOR; BIOLOGICAL-SYSTEMS; ZINPYR FAMILY; ZINC SENSORS; ZN2+; CHEMISTRY; PLATFORM; PROBE; BENZENETHIOLS; DERIVATIVES;
D O I：
10.1016/j.ica.2013.11.033
中图分类号：
O61 [无机化学];
学科分类号：
070301 ; 081704 ;
摘要：
Two new borondipyrromethene-based probes BODIPY1 and BODIPY2 were synthesized and evaluated. The chelators in the two probes, 8-aminoquinoline (AQ) and sulfur function, coordinate to Zn2+ in a synergic manner, thus the change in oxidation state of sulfur function (thioether to sulfoxide) would have sufficient effect on the photophysical response properties. As expected, both BODIPY1 and BODIPY2 display distinct fluorescence enhancement toward Zn2+. However, BODIPY1 and BODIPY2 show different binding properties. Pb2+ interferes with Zn2+ detection in BODIPY1 while has little influence on the fluorescence of BODIPY2, interfering that change of the oxidation state of the sulfur atom from thioether to sulfoxide benefits the Zn2+ -specific fluorescence response. (c) 2013 Elsevier B.V. All rights reserved.
引用
收藏
页码：32 / 37
页数：6
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