X-ray spectroscopy for chemical and energy sciences: the case of heterogeneous catalysis

被引:15
作者
Frenkel, Anatoly I. [1 ]
van Bokhoven, Jeroen A. [2 ,3 ]
机构
[1] Yeshiva Univ, Dept Phys, New York, NY 10016 USA
[2] ETH, Dept Chem & Bioengn, CH-8093 Zurich, Switzerland
[3] Paul Scherrer Inst, Lab Catalysis & Sustainable Chem, CH-5232 Villigen, Switzerland
关键词
heterogeneous catalysis; diffraction-limited storage rings; single-particle spectroscopy; time resolved; X-ray absorption; X-ray emission; IN-SITU; PHOTOSYSTEM-II; BOND-LENGTH; ABSORPTION; NANOPARTICLES; OXIDATION; IDENTIFICATION; ADSORPTION; REACTIVITY; PLATINUM;
D O I
10.1107/S1600577514014854
中图分类号
TH7 [仪器、仪表];
学科分类号
0804 ; 080401 ; 081102 ;
摘要
Heterogeneous catalysis is the enabling technology for much of the current and future processes relevant for energy conversion and chemicals synthesis. The development of new materials and processes is greatly helped by the understanding of the catalytic process at the molecular level on the macro/micro-kinetic time scale and on that of the actual bond breaking and bond making. The performance of heterogeneous catalysts is inherently the average over the ensemble of active sites. Much development aims at unravelling the structure of the active site; however, in general, these methods yield the ensemble-average structure. A benefit of X-ray-based methods is the large penetration depth of the X-rays, enabling in situ and operando measurements. The potential of X-ray absorption and emission spectroscopy methods (XANES, EXAFS, HERFD, RIXS and HEROS) to directly measure the structure of the catalytically active site at the single nanoparticle level using nanometer beams at diffraction-limited storage ring sources is highlighted. The use of pump-probe schemes coupled with single-shot experiments will extend the time range from the micro/macro-kinetic time domain to the time scale of bond breaking and making.
引用
收藏
页码:1084 / 1089
页数:6
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