Hydrodynamics of Trickle Bed Reactors with Catalyst Support Particle Size Distributions

被引:9
作者
Honda, Gregory S. [1 ]
Gase, Philip [1 ]
Hickman, Daniel A. [2 ]
Varma, Arvind [1 ]
机构
[1] Purdue Univ, Sch Chem Engn, W Lafayette, IN 47907 USA
[2] Dow Chem Co USA, Engn & Proc Sci, Midland, MI 48674 USA
关键词
PRESSURE-DROP; LIQUID HOLDUP; FLOW-THROUGH; MODEL; EQUATION;
D O I
10.1021/ie403491x
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Characterization of the hydrodynamics enables operation of trickle bed reactors within the desired flow regime and under conditions for uniform distribution of gas and liquid, resulting in an essentially plug flow contacting pattern. Studies reported in the literature are typically restricted to systems of beds packed with catalyst supports of a uniform size. This work addresses the impact of supports with particle size distributions on reactor hydrodynamics. An experimental database of pressure drop and liquid holdup was developed and, by careful definition of the particle diameter, literature models were adapted to account for the particle size distribution. The resulting models give improved predictions for packing media with a particle size distribution while maintaining applicability to uniform systems.
引用
收藏
页码:9027 / 9034
页数:8
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