Functionalized Thiophene-Based [7]Helicene: Chirooptical Properties versus Electron Delocalization

被引:53
作者
Rajca, Andrzej [1 ]
Pink, Maren [2 ]
Xiao, Shuzhang [1 ]
Miyasaka, Makoto [1 ]
Rajca, Suchada [1 ]
Das, Kausik [1 ]
Plessel, Kristin [1 ]
机构
[1] Univ Nebraska, Dept Chem, Lincoln, NE 68588 USA
[2] Indiana Univ, Dept Chem, IUMSC, Bloomington, IN 47405 USA
基金
美国国家科学基金会;
关键词
CROSS-CONJUGATED OLIGOTHIOPHENES; ASYMMETRIC-SYNTHESIS; OPTICAL-PROPERTIES; CHIROPTICAL PROPERTIES; BAND-GAP; HELICENES; ABSORPTION; RESOLUTION; SYSTEMS; ROUTE;
D O I
10.1021/jo901769c
中图分类号
O62 [有机化学];
学科分类号
070303 ; 081704 ;
摘要
The functionalized, enantiomerically pure [7]helicene 1 derived from bis(benzodithiophene) functionalized with four heptyl groups is prepared from 1,8-dibromo-4,5-diheptylbenzo[1,2-b:4,3-b']dithiophene building block 2. Such [7]helicene structure, functionalized with bromines at the terminal positions of the helicene inner rim and multiple solubilizing alkyl groups, is an attractive building block for long [n]helicenes and oligo[7]helicenes. Chirooptical properties and the degree of electron delocalization are determined and compared to those of analogous carbon-sulfur [7]helicene and [7]helicenes derived from benzodithiophene to provide a correlation between chirooptical properties and the degree of electron delocalization. [7]Helicene 1 possesses a moderately increased electron delocalization, but its chirooptical properties are similar to those for analogous [7]helicenes with relatively lower electron delocalization, indicating that chirooptical properties are not significantly affected by electron delocalization for this series of [7]helicenes. Molecular structures of racemic [7]helicene 1 and its benzodithiophene building block 2 are confirmed by single-crystal X-ray analysis. Crystals of 2 are chiral and adopt the shape of long, flexible, flat needles that can be readily bent.
引用
收藏
页码:7504 / 7513
页数:10
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