Measurement of natural radioactivity and radiation hazards for some natural and artificial building materials available in Romania

As building materials are known to be the second source regarding high radon concentrations, it is very important to determine the amounts of natural radionuclides from every building material in use. In the present study the most frequently used Romanian natural (sand, gypsum, limestone) and artificial (portland cement, lime, clinker, electrofilter powder, fly ash, cement-lime plaster mortar, cement plaster mortar) building materials were analyzed. The absorbed dose rate and the annual effective dose equivalent rate for people living in dwelling buildings made of these building materials under investigation were also calculated. The analysis was performed with gamma-ray spectrometry, with two hyper-pure germanium detectors. The activity concentrations of natural radionuclides were in the ranges: 5.2-511.8 Bq kg(-1) for Ra-226; 0.6-92.6 Bq kg(-1) for Th-232 and < 1-1,720.7 Bq kg(-1) for K-40, respectively. The radium equivalent activity in the fifty-one (51) samples varied from 9 to 603 Bq kg(-1). By calculating all the radioactivity indices (Ra-eq, H (ext), I (alpha), I (yr)) it was found that all the building materials under investigation can be used to erect dwelling buildings. Except for sample SA6, SA7 and SA11 among the natural building materials and sample SG1, SG2, FAH1, CLM1, CM1 among the artificial building materials that are considered hazardous materials when are used in large quantities.