Universal Electrode Interface for Electrocatalytic Oxidation of Liquid Fuels

被引:39
作者
Liao, Hualing [1 ]
Qiu, Zhipeng [1 ]
Wan, Qijin [1 ]
Wang, Zhijie [1 ]
Liu, Yi [1 ]
Yang, Nianjun [1 ,2 ]
机构
[1] Wuhan Inst Technol, Sch Chem & Environm Engn, Wuhan 430073, Hubei, Peoples R China
[2] Univ Siegen, Inst Mat Engn, D-57076 Siegen, Germany
基金
中国国家自然科学基金;
关键词
electrocatalytic oxidation; liquid fuels; carbon nanotubes; palladium nanoparticles; reaction mechanism; oxidation efficiency; fuel cells; FORMIC-ACID ELECTROOXIDATION; WALLED CARBON NANOTUBES; PALLADIUM NANOPARTICLES; METHANOL OXIDATION; ETHANOL OXIDATION; ALCOHOL OXIDATION; PD NANOPARTICLES; ALKALINE MEDIA; PLATINUM NANOPARTICLES; METAL NANOPARTICLES;
D O I
10.1021/am504926r
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Electrocatalytic oxidations of liquid fuels from alcohols, carboxylic acids, and aldehydes were realized on a universal electrode interface. Such an interface was fabricated using carbon nanotubes (CNTs) as the catalyst support and palladium nanoparticles (Pd NPs) as the electrocatalysts. The Pd NPs/CNTs nanocomposite was synthesized using the ethylene glycol reduction method. It was characterized using transmission electron microscopy, energy dispersive X-ray spectroscopy, X-ray diffraction, voltammetry, and impedance. On the Pd NPs/CNTs nanocomposite coated electrode, the oxidations of those liquid fuels occur similarly in two steps: the oxidations of freshly chemisorbed species in the forward (positive-potential) scan and then, in the reverse scan (negative-potential), the oxidations of the incompletely oxidized carbonaceous species formed during the forward scan. The oxidation charges were adopted to study their oxidation mechanisms and oxidation efficiencies. The oxidation efficiency follows the order of aldehyde (formaldehyde) > carboxylic acid (formic acid) > alcohols (ethanol > methanol > glycol > propanol). Such a Pd NPs/CNTs nanocomposite coated electrode is thus promising to be applied as the anode for the facilitation of direct fuel cells.
引用
收藏
页码:18055 / 18062
页数:8
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