The tunable quantum spin ladder Cu(Qnx)(Cl(1-x)Brx)2

被引:8
作者
Povarov, K. Yu. [1 ,3 ]
Lorenz, W. E. A. [1 ]
Xiao, F. [2 ]
Landee, C. P. [2 ]
Krasnikova, Y. [3 ,4 ]
Zheludev, A. [1 ]
机构
[1] Swiss Fed Inst Technol, Solid State Phys Lab, Zurich, Switzerland
[2] Clark Univ, Dept Phys, Worcester, MA 01610 USA
[3] RAS, PL Kapitza Inst Phys Problems, Moscow 119334, Russia
[4] Moscow Inst Phys & Technol, Dolgoprudnyi 141700, Russia
关键词
Spin ladders; Bond disorder; MAGNETS;
D O I
10.1016/j.jmmm.2014.06.060
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We report magnetic, specific heat and ESR measurements on a series of S=1/2 spin ladder compounds Cu(Qnx)(Cl(1-x)Brx)(2). Down to T=2 K all the observables can be described by the spin ladder model with about 1% of S=1/2 impurities in the background, which are present even in a nominally pure Cu(Qnx)Cl-2 and Cu(Qnx)Br-2, for the whole range of 0 <= x <= 1. We extract ladder exchange constants J(l)(x) and J(r)(x) as well as the gap value Delta(x) by comparing the experimental data to quantum Monte-Carlo simulations. As the ESR measurements show the g-factor of impurities to be precisely equal to g-factor of the ladder spins, we suppose the impurities to be the consequence of structural defects resulting in broken ladder ends. (C) 2014 Elsevier B.V. All rights reserved.
引用
收藏
页码:62 / 67
页数:6
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