Lattice Boltzmann simulations of anisotropic permeabilities in carbon paper gas diffusion layers

被引:204
作者
Hao, Liang [1 ,2 ]
Cheng, Ping [1 ,2 ]
机构
[1] Shanghai Jiao Tong Univ, Minist Educ, Key Lab Power Machinery & Engn, Shanghai 200240, Peoples R China
[2] Shanghai Jiao Tong Univ, Sch Mech & Power Engn, Shanghai 200240, Peoples R China
基金
中国国家自然科学基金;
关键词
Lattice Boltzmann; Permeability; Gas diffusion layer; Anisotropic; Tortuosity; FUEL-CELL; FLOW SIMULATION; MODEL; TRANSPORT; ELECTRODE; MEDIA; PERFORMANCE; POROSITY; INPLANE;
D O I
10.1016/j.jpowsour.2008.09.086
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The multiple-relaxation-time (MRT) lattice Boltzmann method (LBM) with multi-reflection solid boundary conditions is used to study anisotropic permeabilities of a carbon paper gas diffusion layer (GDL) in a fuel cell. The carbon paper is reconstructed using the stochastic method, in which various porosities and microstructures are achieved to simulate different samples. The simulated permeability and tortuosity show anisotropic characteristics of the reconstructed carbon papers with in-plane permeability higher than through-plane, and in-plane tortuosity lower than through-plane. The calculated permeabilities are in good agreement with existing measurements. The relationship between the permeability and the porosity is fitted with empirical relations and some fitting constants are determined. Furthermore, the obtained relationship of tortuosity and porosity is used in a fractal model for permeabilities. The results indicate that the fractal model and the Kozeny-Carman equation provide similar predictions on the through-plane permeability of the carbon paper GDL. (c) 2008 Published by Elsevier B.V.
引用
收藏
页码:104 / 114
页数:11
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