Identification of Sources of Fine Particulate Matter in Kandy, Sri Lanka

被引:13
作者
Seneviratne, Shirani [1 ]
Handagiripathira, Lakmali [1 ]
Sanjeevani, Sisara [1 ]
Madusha, Dulanjalee [1 ]
Waduge, Vajira Ariyaratna Ariyaratna [1 ]
Attanayake, Thilaka [1 ]
Bandara, Deepthi [2 ]
Hopke, Philip K. [3 ]
机构
[1] Atom Energy Board, 60-460 Baseline Rd, Orugodawatta, Wellampitiya, Sri Lanka
[2] Cent Environm Author, Battaramulla, Sri Lanka
[3] Clarkson Univ, Ctr Air Resources Engn & Sci, Potsdam, NY 13699 USA
关键词
Particulate matter; Source apportionment; Positive Matrix Factorization; Sri Lanka; ATMOSPHERIC AEROSOL; AIR-POLLUTION; URBAN; PARTICLES; COLOMBO; SITES; DHAKA; AREAS; SMOKE; DELHI;
D O I
10.4209/aaqr.2016.03.0123
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Kandy is the second largest city in Sri Lanka and a major tourist destination. It is a fast growing city with continuous construction of buildings, roads and historical places. More than 100 samples of fine particulate matter (PM) were collected using a GENT stacked filter sampler from a fixed site at the regional sampling station of Department of Meteorology situated in Katugastota, Kandy over the period of 2012 to 2014. Black carbon (BC) in these filters were determined by reflectance measurements while their elemental compositions were determined using the X-ray fluorescence spectrometry. Analysis of the elemental data suggests that the PM in Kandy originates largely from re-suspended soil and anthropogenic sources. The fine particulate matter data including BC and major elements (Na, Mg, Al, Si, Cl, Fe, Zn, Ni, Cu, V, S, Br, Pb, Cr, K, Ca and Ti) was analyzed using EPA-PMF version 5.0 (Positive Matrix Factorization) to explore the possible sources of the PM at the study site. Five factors were found and identified as soil, aged sea salt, vehicular emissions, biomass burning, and industrial sources.
引用
收藏
页码:476 / 484
页数:9
相关论文
共 33 条
[1]  
Begum B.A., 2006, Aerosol and Air Quality Research, V6, P334, DOI [10.4209/aaqr.2006.12.0001, DOI 10.4209/AAQR.2006.12.0001]
[2]   Investigation of sources of atmospheric aerosol at a hot spot area in Dhaka, Bangladesh [J].
Begum, BA ;
Biswas, SK ;
Kim, E ;
Hopke, PK ;
Khaliquzzaman, M .
JOURNAL OF THE AIR & WASTE MANAGEMENT ASSOCIATION, 2005, 55 (02) :227-240
[3]   Investigation of sources of atmospheric aerosol at urban and semi-urban areas in Bangladesh [J].
Begum, BA ;
Kim, E ;
Biswas, SK ;
Hopke, PK .
ATMOSPHERIC ENVIRONMENT, 2004, 38 (19) :3025-3038
[4]   Long-range transport of soil dust and smoke pollution in the South Asian region [J].
Begum, Bilkis A. ;
Biswas, Swapan K. ;
Pandit, Gauri G. ;
Saradhi, I. Vijaya ;
Waheed, Shahida ;
Siddique, Naila ;
Seneviratne, M. C. Shirani ;
Cohen, David D. ;
Markwitz, Andreas ;
Hopke, Philip K. .
ATMOSPHERIC POLLUTION RESEARCH, 2011, 2 (02) :151-157
[5]   Impact of unleaded gasoline introduction on the concentration of lead in the air of Dhaka, Bangladesh [J].
Biswas, SK ;
Tarafdar, SA ;
Islam, A ;
Khaliquzzaman, M ;
Tervahattu, H ;
Kupiainen, K .
JOURNAL OF THE AIR & WASTE MANAGEMENT ASSOCIATION, 2003, 53 (11) :1355-1362
[6]   Investigation of sources of atmospheric aerosol at urban and suburban residential areas in Thailand by positive matrix factorization [J].
Chueinta, W ;
Hopke, PK ;
Paatero, P .
ATMOSPHERIC ENVIRONMENT, 2000, 34 (20) :3319-3329
[7]  
Cohen D.D., 1997, STUDY FINE ATMOSPHER
[8]   Characterisation and source apportionment of fine particulate sources at Hanoi from 2001 to 2008 [J].
Cohen, David D. ;
Crawford, Jagoda ;
Stelcer, Eduard ;
Bac, Vuong Thu .
ATMOSPHERIC ENVIRONMENT, 2010, 44 (03) :320-328
[9]   AN ASSOCIATION BETWEEN AIR-POLLUTION AND MORTALITY IN 6 UNITED-STATES CITIES [J].
DOCKERY, DW ;
POPE, CA ;
XU, XP ;
SPENGLER, JD ;
WARE, JH ;
FAY, ME ;
FERRIS, BG ;
SPEIZER, FE .
NEW ENGLAND JOURNAL OF MEDICINE, 1993, 329 (24) :1753-1759
[10]   PARTICULATE AIR-POLLUTANTS - A COMPARISON OF BRITISH SMOKE WITH OPTICAL-ABSORPTION COEFFICIENT AND ELEMENTAL CARBON CONCENTRATION [J].
EDWARDS, JD ;
OGREN, JA ;
WEISS, RE ;
CHARLSON, RJ .
ATMOSPHERIC ENVIRONMENT, 1983, 17 (11) :2337-2341