Evaluation of synergistic effect from Ag-AgCl1/3Br1/3I1/3 composite on photocatalytic degradation the oil field pollutants

被引:5
作者
Zhang, Xu [1 ]
Yang, Ping [2 ,3 ]
Yang, Bo [4 ]
Bai, Yang [3 ]
Liu, Weihua [1 ]
Zhang, Yi [5 ,6 ]
机构
[1] Chongqing Univ Sci & Technol, Sch Petr & Nat Gas Engn, Chongqing 401331, Peoples R China
[2] Sichuan Prov Acad Ind Environm Monitoring, Chengdu 610045, Peoples R China
[3] Southwest Petr Univ, Sch Oil & Nat Gas Engn, State Key Lab Oil & Gas Reservoir Geol & Exploita, Chengdu 610500, Peoples R China
[4] Southwest Petr Univ, Coll Elect & Mech Engn, Chengdu 610500, Peoples R China
[5] Natl & Local Joint Engn Res Ctr Shale Gas Explora, Chongqing 401120, Peoples R China
[6] Inst Geol & Mineral Resources, Chongqing 401120, Peoples R China
基金
中国国家自然科学基金;
关键词
Ag-AgCl1/3Br1/3; I-1/3; Synergistic; SPR; Phenol; VISIBLE-LIGHT PHOTOCATALYSTS; SURFACE-PLASMON RESONANCE; IN-SITU SYNTHESIS; FACILE SYNTHESIS; AG/AGX X; AG; BR; CL; HETEROJUNCTION; NANOCOMPOSITE;
D O I
10.1016/j.saa.2020.119029
中图分类号
O433 [光谱学];
学科分类号
0703 ; 070302 ;
摘要
A series of Ag/AgX (X = Cl, Br, I; X = Cl, Br, or X = Cl, I, or X = Br, I; X = Cl, Br, and I) composite photocatalysts were synthesized via a facile photoreduction. The several characterization methods of Xray diffraction (XRD), energy dispersive X-ray spectrometry (EDS) mapping and X- ray photoelectron spectroscopy ( XPS) were characterized the samples. Through evaluation the photocatalytic activity of degradation rhodamine, methyl orange, and phenol, Ag- AgCl1/3Br1/3I1/3 exhibited the superior selective photocatalytic activities than other photocatalysts. The reason for improved photocatalytic property of Ag- AgCl1/3Br1/3I1/3 was attributed to the multifarious halogen atoms with the synergistic effect and the surface plasmon resonance (SPR) effect of Ag-0. Furthermore, the recycle experiments were conducted to reveal the stability and reusability, the trapping experiments confirmed the active species of AgAgCl1/3Br1/3I1/3. (C) 2020 Published by Elsevier B.V.
引用
收藏
页数:10
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