Remarkable visible-light induced hydrogen generation with ZnIn2S4 microspheres/CuInS2 quantum dots photocatalytic system

被引：53
作者：
Cavdar, Onur [1 ]
Malankowska, Anna [1 ]
Amgar, Daniel [2 ]
Mazierski, Pawel [1 ]
Luczak, Justyna [3 ]
Lisowski, Wojciech [4 ]
Zaleska-Medynska, Adriana [1 ]
机构：
[1] Univ Gdansk, Fac Chem, Dept Environm Technol, PL-80308 Gdansk, Poland
[2] Weizmann Inst Sci, Dept Phys Complex Syst, Fac Phys, IL-761000 Rehovot, Israel
[3] Gdansk Univ Technol, Dept Proc Engn & Chem Technol, Fac Chem, PL-80233 Gdansk, Poland
[4] Polish Acad Sci, Inst Phys Chem, PL-01224 Warsaw, Poland
来源：
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY | 2021年 / 46卷 / 01期
关键词：
REDUCED GRAPHENE OXIDE; LIGAND-EXCHANGE; H-2; PRODUCTION; EFFICIENT; WATER; TIO2; EVOLUTION; CDS; NANOSHEETS; NANOPARTICLES;
D O I：
10.1016/j.ijhydene.2020.09.212
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
A new and active material in the form of ZnIn2S4 microspheres decorated by CuInS2 quantum dots have been obtained by hydrothermal method for the first time. The optimum amount of CuInS2 quantum dots (1.13 wt.%) introduced into rection medium during ZnIn2S4 microspheres synthesis increased the photocatalytic H-2 generation rate by 2.5 times than that of bare ZnIn2S4 photocatalysis under visible light irradiation. This sample exhibited strong photoactivity in the extended visible range up to 540 nm with 30.6% apparent quantum efficiency (lambda = 420 nm). (C) 2020 The Authors. Published by Elsevier Ltd on behalf of Hydrogen Energy Publications LLC.
引用
收藏
页码：486 / 498
页数：13
相关论文
共 78 条
[1]   Luminescence and stability of aqueous thioalkyl acid capped CdSe/ZnS quantum dots correlated to ligand ionization [J].
Algar, W. Russ ;
Krull, Ulrich J. .
CHEMPHYSCHEM, 2007, 8 (04) :561-568
[2]   Hierarchical SrTiO3/TiO2 nanofibers heterostructures with high efficiency in photocatalytic H2 generation [J].
Bai, Hongwei ;
Juay, Jermyn ;
Liu, Zhaoyang ;
Song, Xiaoxiao ;
Lee, Siew Siang ;
Sun, Darren Delai .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2012, 125 :367-374
[3]   Quantum dot-decorated semiconductor micro- and nanoparticles: A review of their synthesis, characterization and application in photocatalysis [J].
Bajorowicz, Beata ;
Kobylanski, Marek P. ;
Golabiewska, Anna ;
Nadolna, Joanna ;
Zaleska-Medynska, Adriana ;
Malankowska, Anna .
ADVANCES IN COLLOID AND INTERFACE SCIENCE, 2018, 256 :352-372
[4]   Self-templated synthesis of nanoporous CdS nanostructures for highly efficient photocatalytic hydrogen production under visible [J].
Bao, Ningzhong ;
Shen, Liming ;
Takata, Tsuyoshi ;
Domen, Kazunari .
CHEMISTRY OF MATERIALS, 2008, 20 (01) :110-117
[5]   Quantum Dots and Their Multimodal Applications: A Review [J].
Bera, Debasis ;
Qian, Lei ;
Tseng, Teng-Kuan ;
Holloway, Paul H. .
MATERIALS, 2010, 3 (04) :2260-2345
[6]   Resolving surface chemical states in XPS analysis of first row transition metals, oxides and hydroxides: Sc, Ti, V, Cu and Zn [J].
Biesinger, Mark C. ;
Lau, Leo W. M. ;
Gerson, Andrea R. ;
Smart, Roger St. C. .
APPLIED SURFACE SCIENCE, 2010, 257 (03) :887-898
[7]  
Booth Matthew., 2014, Synthesis and Characterisation of CuInS 2 Quantum Dots
[8]   Green chemistry approach for the synthesis of ZnO-carbon dots nanocomposites with good photocatalytic properties under visible light [J].
Bozetine, Hakima ;
Wang, Qi ;
Barras, Alexandre ;
Li, Musen ;
Hadjersi, Toufik ;
Szunerits, Sabine ;
Boukherroub, Rabah .
JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2016, 465 :286-294
[9]   Layered Platinum Dichalcogenides (PtS2, PtSe2, and PtTe2) Electrocatalysis: Monotonic Dependence on the Chalcogen Size [J].
Chia, Xinyi ;
Adriano, Ambrosi ;
Lazar, Petr ;
Sofer, Zdenek ;
Luxa, Jan ;
Pumera, Martin .
ADVANCED FUNCTIONAL MATERIALS, 2016, 26 (24) :4306-4318
[10]   Synthesis, Characterization, and Growth Mechanism of n-Type CuInS2 Colloidal Particles [J].
Courtel, Fabrice M. ;
Paynter, Royston W. ;
Marsan, Benoit ;
Morin, Mario .
CHEMISTRY OF MATERIALS, 2009, 21 (16) :3752-3762
12345678