Ammonia-induced robust photocatalytic hydrogen evolution of graphitic carbon nitride

被引:115
作者
Yang, Pengju [1 ,2 ]
Zhao, Jianghong [1 ]
Qiao, Wei [1 ,2 ]
Li, Li [1 ]
Zhu, Zhenping [1 ]
机构
[1] Chinese Acad Sci, Inst Coal Chem, State Key Lab Coal Convers, Taiyuan 030001, Peoples R China
[2] Univ Chinese Acad Sci, Beijing 100039, Peoples R China
关键词
VISIBLE-LIGHT; NANOSHEETS; PHOTOSYNTHESIS; SEMICONDUCTORS; CATALYSTS; ELECTRODE; WATER; UREA; SOFT;
D O I
10.1039/c5nr05570a
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
We report a new and effective method to prepare high activity graphitic carbon nitride (g-C3N4) by a simple ammonia etching treatment. The obtained g-C3N4 displays a high BET surface area and enhanced electron/hole separation efficiency. The hydrogen evolution rates improved from 52 mu mol h(-1) to 316.7 mu mol h(-1) under visible light.
引用
收藏
页码:18887 / 18890
页数:4
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