Modeling and Experimental Study of CO2 Removal by Alkanolamines in a Packed Bed

被引:3
|
作者
Rahimi, Amir [1 ]
Tavakoli, Touraj [1 ]
Saadat, Amin [1 ]
Niksiar, Arezou [2 ]
机构
[1] Univ Isfahan, Dept Chem Engn, Coll Engn, Esfahan 8174673441, Iran
[2] Amirkabir Univ Technol, Dept Chem Engn, Tehran, Iran
关键词
alkanolamines; carbon dioxide; packed bed; reactive absorption; CARBON-DIOXIDE ABSORPTION; AQUEOUS-SOLUTIONS; GAS-ABSORPTION; MONOETHANOLAMINE; KINETICS; SOLUBILITY; DIFFUSIVITY; N2O;
D O I
10.1080/01496395.2013.845849
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Absorption of CO2 by monoethanolamine, diethanolamine, and triethanolamine solutions in a lab-scale packed bed tower was investigated. A model for analyzing the heat and mass transfer mechanism in the presence of reaction was developed and validated using the measured data for MEA and TEA solutions and the results were compared with the others' experimental data. The well-known correlations for determining Henry's constant, as a critical parameter in the presented model, were evaluated and it was shown that the available correlations are often limited to a narrow range of operating conditions which could limit the applicability of the available models.
引用
收藏
页码:317 / 328
页数:12
相关论文
共 50 条
  • [41] Experimental and rate-based modeling study of CO2 capture by aqueous monoethanolamine
    Li, Xiaofei
    Wang, Shujuan
    Chen, Changhe
    GREENHOUSE GASES-SCIENCE AND TECHNOLOGY, 2014, 4 (04): : 495 - 508
  • [42] CO2 Capture Using Solutions of Alkanolamines and Aminosilicones
    Perry, Robert J.
    Davis, Jason L.
    ENERGY & FUELS, 2012, 26 (04) : 2512 - 2517
  • [43] Capture of CO2 by highly concentrated alkanolamine solutions in a rotating packed bed
    Wang, Yi-Ming
    Chen, Yu-Shao
    ENVIRONMENTAL PROGRESS & SUSTAINABLE ENERGY, 2019, 38 (06)
  • [44] Study of novel solvent for CO2 post-combustion capture
    Hadri, Nabil E. L.
    Dang Viet Quang
    Abu-Zahra, Mohammad R. M.
    CLEAN, EFFICIENT AND AFFORDABLE ENERGY FOR A SUSTAINABLE FUTURE, 2015, 75 : 2268 - 2286
  • [45] CFD Modeling of Reactive Absorption of CO2 by Aqueous MEA Solution in a Rotating Packed Bed
    Zhang, Wei
    Zhang, Weiwen
    Li, Xinyang
    Fu, Cheng
    Huang, Bin
    Li, Yuxing
    Xie, Peng
    ENERGY & FUELS, 2024, 38 (14) : 13104 - 13114
  • [46] Physical properties of PZ solution used as a solvent for CO2 removal
    Moioli, Stefania
    Pellegrini, Laura A.
    CHEMICAL ENGINEERING RESEARCH & DESIGN, 2015, 93 : 720 - 726
  • [47] Industrial Applied and Modeling Research on Selective H2S Removal Using a Rotating Packed Bed
    Qian, Zhi
    Li, Zhen-Hu
    Guo, Kai
    INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2012, 51 (23) : 8108 - 8116
  • [48] Modeling CO2 absorption into concentrated aqueous monoethanolamine and piperazine
    Dugas, Ross E.
    Rochelle, Gary T.
    CHEMICAL ENGINEERING SCIENCE, 2011, 66 (21) : 5212 - 5218
  • [49] Experimental investigation of a packed bed membrane reactor for the direct conversion of CO2 to dimethyl ether
    Poto, Serena
    Tanco, Margot Annabell Llosa
    Tanaka, David Alfredo Pacheco
    d'Angelo, M. Fernanda Neira
    Gallucci, Fausto
    JOURNAL OF CO2 UTILIZATION, 2023, 72
  • [50] A novel methodology for the modeling of CO2 absorption in monoethanolamine (MEA) using discrimination of rival kinetics
    Hiwale, Rameshwar
    Smith, Robin
    Hwang, Sungwon
    JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY, 2015, 25 : 78 - 88