A novel method for extracting oscillator strength of select rare-earth ion optical transitions in nanostructured dielectric materials

被引:16
|
作者
Muenchausen, R. E. [1 ]
Jacobsohn, L. G. [1 ]
Bennett, B. L. [1 ]
McKigney, E. A. [1 ]
Smith, J. F. [1 ]
Cooke, D. W. [1 ]
机构
[1] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA
关键词
nanophosphor; rare earth; oscillator strength; photoluminescence;
D O I
10.1016/j.ssc.2006.07.022
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
A new technique to obtain the oscillator strength of select rare-earth optical transitions in nanostructured dielectric materials (nanophosphors) is presented. It is based on the experimentally observed nanophosphor lifetime dependence on the embedding medium. A constant oscillator strength and parity-allowed electric dipole transitions of the RE ion emission are assumed. The oscillator strength is obtained from the slope of the 1/tau(ij) vs. n(n(2) + 2)(2) plot, where tau(ij) is the radiative lifetime of transition between states i and j, and n is the index of refraction of the embedding medium. The use of the technique is illustrated for the Y2SiO5:Ce nanophosphor. (c) 2006 Elsevier Ltd. All rights reserved.
引用
收藏
页码:497 / 500
页数:4
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