Pump-probe femtosecond-laser VUV REMPI technique applied to the study of highly excited states of allyl iodide

被引:5
作者
Baklanov, AV
Maltsev, VP
Karlsson, L
Sassenberg, U
Persson, A
机构
[1] UNIV STOCKHOLM,DEPT PHYS,S-11385 STOCKHOLM,SWEDEN
[2] LUND INST TECHNOL ATOM PHYS,S-22100 LUND,SWEDEN
来源
JOURNAL OF THE CHEMICAL SOCIETY-FARADAY TRANSACTIONS | 1996年 / 92卷 / 10期
关键词
D O I
10.1039/ft9969201681
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The pump-probe REMPI technique has been used for a study of the femtosecond dynamics of the allyl iodide (Al) molecule excited in the VUV region. The VUV radiation was produced by non-resonant quintupling of Ti:S laser radiation in the mercury vapour or xenon gas. The lifetime of the excited state (hv approximate to 7.8 eV) of AI was found to be 290 +/- 30 fs. The nature of the process governing this decay time is discussed.
引用
收藏
页码:1681 / 1682
页数:2
相关论文
共 15 条
[1]   DYNAMICS OF VERY HIGH RYDBERG STATES OF AROMATIC-MOLECULES [J].
BAHATT, D ;
EVEN, U ;
LEVINE, RD .
JOURNAL OF CHEMICAL PHYSICS, 1993, 98 (02) :1744-1747
[2]   RESONANT 2-PHOTON IONIZATION DETECTION OF ATOMIC IODINE RESULTING FROM PHOTODISSOCIATION OF ALLYL IODIDE UNDER VIBRATIONAL (C-H OVERTONE) EXCITATION [J].
BAKLANOV, AV ;
MALTSEV, VP ;
KARLSSON, L ;
LINDGREN, B ;
SASSENBERG, U .
CHEMICAL PHYSICS, 1994, 184 (1-3) :357-363
[3]   LIFETIME OF THE S(3) STATE OF CS2 MEASURED BY FEMTOSECOND ULTRAVIOLET MULTIPHOTON IONIZATION SPECTROSCOPY [J].
BARONAVSKI, AP ;
OWRUTSKY, JC .
CHEMICAL PHYSICS LETTERS, 1994, 221 (5-6) :419-425
[4]   THE STRUCTURE OF THE MOLECULAR ION OF ALLYL BROMIDE [J].
CARRUPT, PA ;
RIVEROS, JM ;
STAHL, D .
INTERNATIONAL JOURNAL OF MASS SPECTROMETRY AND ION PROCESSES, 1991, 110 (1-2) :R1-R5
[5]   KINETIC-ENERGY, FEMTOSECOND RESOLVED REACTION DYNAMICS - MODES OF DISSOCIATION (IN IODOBENZENE) FROM TIME-VELOCITY CORRELATIONS [J].
CHENG, PY ;
ZHONG, D ;
ZEWAIL, AH .
CHEMICAL PHYSICS LETTERS, 1995, 237 (5-6) :399-405
[6]   LIFETIMES OF VERY HIGH RYDBERG STATES OF AROMATIC-MOLECULES [J].
CHUPKA, WA .
JOURNAL OF CHEMICAL PHYSICS, 1993, 99 (08) :5800-5806
[7]   FEMTOSECOND REAL-TIME PROBING OF REACTIONS .14. RYDBERG STATES OF METHYL-IODIDE [J].
GUO, H ;
ZEWAIL, AH .
CANADIAN JOURNAL OF CHEMISTRY-REVUE CANADIENNE DE CHIMIE, 1994, 72 (03) :947-957
[8]  
HARRIS CB, 1990, SPRINGER SERIES C 12, V53
[9]  
Hilbig R., 1986, Comments on Atomic and Molecular Physics, V18, P157
[10]   FEMTOSECOND REACTION DYNAMICS OF RYDBERG STATES - METHYL-IODIDE [J].
JANSSEN, MHM ;
DANTUS, M ;
GUO, H ;
ZEWAIL, AH .
CHEMICAL PHYSICS LETTERS, 1993, 214 (3-4) :281-289