Ultra-light, compressible and fire-resistant graphene aerogel as a highly efficient and recyclable absorbent for organic liquids

被引:374
作者
Li, Jihao [1 ,2 ,3 ]
Li, Jingye [1 ,2 ]
Meng, Hu [1 ,2 ,3 ]
Xie, Siyuan [1 ,2 ,3 ]
Zhang, Bowu [1 ,2 ]
Li, Linfan [1 ,2 ]
Ma, Hongjuan [1 ,2 ]
Zhang, Jianyong [1 ,2 ]
Yu, Ming [1 ,2 ]
机构
[1] Chinese Acad Sci, TMSR Res Ctr, Shanghai 201800, Peoples R China
[2] Chinese Acad Sci, CAS Key Lab Nucl Radiat & Nucl Energy Technol, Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China
[3] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
基金
中国国家自然科学基金;
关键词
CARBON; OXIDE; NANOCOMPOSITES; RESORCINOL; SORPTION; SORBENT; PERFORMANCE; POLLUTANTS; DESIGN; SILICA;
D O I
10.1039/c3ta14725h
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Compressive graphene aerogels were obtained by the one-step reduction and self-assembly of graphene oxide with ethylenediamine and then freeze-drying. The aerogels hold good compressibility, variable electrical resistance and fire-resistance. The high porosity with a hydrophobic nature, allows the aerogels to absorb different organic liquids, and the absorption-squeezing process has been demonstrated for oil collection.
引用
收藏
页码:2934 / 2941
页数:8
相关论文
共 57 条
[1]   Preparation and properties of resorcinol-formaldehyde organic and carbon gels [J].
Al-Muhtaseb, SA ;
Ritter, JA .
ADVANCED MATERIALS, 2003, 15 (02) :101-+
[2]   Giant-Stroke, Superelastic Carbon Nanotube Aerogel Muscles [J].
Aliev, Ali E. ;
Oh, Jiyoung ;
Kozlov, Mikhail E. ;
Kuznetsov, Alexander A. ;
Fang, Shaoli ;
Fonseca, Alexandre F. ;
Ovalle, Raquel ;
Lima, Marcio D. ;
Haque, Mohammad H. ;
Gartstein, Yuri N. ;
Zhang, Mei ;
Zakhidov, Anvar A. ;
Baughman, Ray H. .
SCIENCE, 2009, 323 (5921) :1575-1578
[3]   Experimental investigation of various vegetable fibers as sorbent materials for oil spills [J].
Annunciado, TR ;
Sydenstricker, THD ;
Amico, SC .
MARINE POLLUTION BULLETIN, 2005, 50 (11) :1340-1346
[4]   Study of oil sorption by expanded perlite at 298.15 K [J].
Bastani, D. ;
Safekordi, A. A. ;
Alihosseini, A. ;
Taghikhani, V. .
SEPARATION AND PURIFICATION TECHNOLOGY, 2006, 52 (02) :295-300
[5]   Oil spill cleanup from sea water by sorbent materials [J].
Bayat, A ;
Aghamiri, SF ;
Moheb, A ;
Vakili-Nezhaad, GR .
CHEMICAL ENGINEERING & TECHNOLOGY, 2005, 28 (12) :1525-1528
[6]   Spongy Graphene as a Highly Efficient and Recyclable Sorbent for Oils and Organic Solvents [J].
Bi, Hengchang ;
Xie, Xiao ;
Yin, Kuibo ;
Zhou, Yilong ;
Wan, Shu ;
He, Longbing ;
Xu, Feng ;
Banhart, Florian ;
Sun, Litao ;
Ruoff, Rodney S. .
ADVANCED FUNCTIONAL MATERIALS, 2012, 22 (21) :4421-4425
[7]   Super-compressible foamlike carbon nanotube films [J].
Cao, AY ;
Dickrell, PL ;
Sawyer, WG ;
Ghasemi-Nejhad, MN ;
Ajayan, PM .
SCIENCE, 2005, 310 (5752) :1307-1310
[8]   In situ self-assembly of mild chemical reduction graphene for three-dimensional architectures [J].
Chen, Wufeng ;
Yan, Lifeng .
NANOSCALE, 2011, 3 (08) :3132-3137
[9]   NATURAL SORBENTS IN OIL-SPILL CLEANUP [J].
CHOI, HM ;
CLOUD, RM .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1992, 26 (04) :772-776
[10]   Extent and frequency of vessel oil spills in US marine protected areas [J].
Dalton, Tracey ;
Jin, Di .
MARINE POLLUTION BULLETIN, 2010, 60 (11) :1939-1945