Selective Conversion of CO2 into para-Xylene over a ZnCr2O4-ZSM-5 Catalyst

被引：43
作者：
Gao, Weizhe [1 ]
Guo, Lisheng [1 ]
Cui, Yu [1 ]
Yang, Guohui [1 ]
He, Yingluo [1 ]
Zeng, Chunyang [2 ]
Taguchi, Akira [3 ]
Abe, Takayuki [3 ]
Ma, Qingxiang [4 ]
Yoneyama, Yoshiharu [1 ]
Tsubaki, Noritatsu [1 ]
机构：
[1] Toyama Univ, Dept Appl Chem, Sch Engn, Gofuku 3190, Toyama 9308555, Japan
[2] China Petr Chem Ind Federat, Beijing 100723, Peoples R China
[3] Toyama Univ, Hydrogen Isotope Res Ctr, Gofuku 3190, Toyama 9308555, Japan
[4] Ningxia Univ, Coll Chem & Chem Engn, State Key Lab High Efficiency Coal Utilizat & Gre, Yinchuan 750021, Ningxia, Peoples R China
来源：
CHEMSUSCHEM | 2020年 / 13卷 / 24期
基金：
日本科学技术振兴机构;
关键词：
aromatics; CO2; conversion; green chemistry; oxide-zeolite catalyst; ZSM-5; zeolite; CARBON-DIOXIDE; LOWER OLEFINS; AROMATICS; METHANOL; SYNGAS; HYDROGENATION;
D O I：
10.1002/cssc.202002305
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
An oxide-zeolite (ZnCr2O4-ZSM-5) catalyst for directly converting CO2 to aromatics was designed and developed. It showed high PX/X (the C-mol ratio of p-xylene to all xylene) and PX/aromatics (the C-mol ratio of p-xylene to aromatics) ratios, which reached 97.3 and 63.9 %, respectively.
引用
收藏
页码：6541 / 6545
页数：5
相关论文
共 24 条
  • [1] Bifunctional Catalysts for One-Step Conversion of Syngas into Aromatics with Excellent Selectivity and Stability
    Cheng, Kang
    Zhou, Wei
    Kang, Jincan
    He, Shun
    Shi, Shulin
    Zhang, Qinghong
    Pan, Yang
    Wen, Wu
    Wang, Ye
    [J]. CHEM, 2017, 3 (02): : 334 - 347
  • [2] Selective Production of Aromatics Directly from Carbon Dioxide Hydrogenation
    Cui, Xu
    Gao, Peng
    Li, Shenggang
    Yang, Chengguang
    Liu, Ziyu
    Wang, Hui
    Zhong, Liangshu
    Sun, Yuhan
    [J]. ACS CATALYSIS, 2019, 9 (05) : 3866 - 3876
  • [3] Direct Production of Lower Olefins from CO2 Conversion via Bifunctional Catalysis
    Gao, Peng
    Dang, Shanshan
    Li, Shenggang
    Bu, Xianni
    Liu, Ziyu
    Qiu, Minghuang
    Yang, Chengguang
    Wang, Hui
    Zhong, Liangshu
    Han, Yong
    Liu, Qiang
    Wei, Wei
    Sun, Yuhan
    [J]. ACS CATALYSIS, 2018, 8 (01): : 571 - 578
  • [4] Sustainable production of light olefins from greenhouse gas CO2 over SAPO-34 supported modified cerium oxide
    Ghasemi, Mostafa
    Mohammadi, Majid
    Sedighi, Mehdi
    [J]. MICROPOROUS AND MESOPOROUS MATERIALS, 2020, 297 (297)
  • [5] GONG Y, 2019, ATMOSPHERE-BASEL, V10, DOI DOI 10.3390/atmos10060302
  • [6] Selective conversion of syngas to light olefins
    Jiao, Feng
    Li, Jinjing
    Pan, Xiulian
    Xiao, Jianping
    Li, Haobo
    Ma, Hao
    Wei, Mingming
    Pan, Yang
    Zhou, Zhongyue
    Li, Mingrun
    Miao, Shu
    Li, Jian
    Zhu, Yifeng
    Xiao, Dong
    He, Ting
    Yang, Junhao
    Qi, Fei
    Fu, Qiang
    Bao, Xinhe
    [J]. SCIENCE, 2016, 351 (6277) : 1065 - 1068
  • [7] Tuning Selectivity of CO2 Hydrogenation Reactions at the Metal/Oxide Interface
    Kattel, Shyam
    Liu, Ping
    Chen, Jingguang G.
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2017, 139 (29) : 9739 - 9754
  • [8] Highly Selective Conversion of Carbon Dioxide to Aromatics over Tandem Catalysts
    Li, Zelong
    Qu, Yuanzhi
    Wang, Jijie
    Liu, Hailong
    Li, Mingrun
    Miao, Shu
    Li, Can
    [J]. JOULE, 2019, 3 (02) : 570 - 583
  • [9] Selective transformation of carbon dioxide into lower olefins with a bifunctional catalyst composed of ZnGa2O4 and SAPO-34
    Liu, Xiaoliang
    Wang, Mengheng
    Zhou, Cheng
    Zhou, Wei
    Cheng, Kang
    Kang, Jincan
    Zhang, Qinghong
    Deng, Weiping
    Wang, Ye
    [J]. CHEMICAL COMMUNICATIONS, 2018, 54 (02) : 140 - 143
  • [10] Direct and selective conversion of methanol to para-xylene over Zn ion doped ZSM-5/silicalite-1 core-shell zeolite catalyst
    Miyake, Koji
    Hirota, Yuichiro
    Ono, Kaito
    Uchida, Yoshiaki
    Tanaka, Shunsuke
    Nishiyama, Norikazu
    [J]. JOURNAL OF CATALYSIS, 2016, 342 : 63 - 66
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