High zinc removal from water and soil using struvite-supported diatomite obtained by nitrogen and phosphate recovery from wastewater

被引:9
作者
Li, Yuan [1 ]
Wang, Xuejiang [2 ]
Xu, Hongbin [1 ]
Xia, Peng [2 ]
Wang, Hao [2 ]
Jing, Huanping [2 ]
Li, Jing [2 ]
Zhao, Jianfu [2 ]
机构
[1] Zhengzhou Univ, Coll Environm & Water Conservancy, Zhengzhou 450001, Henan, Peoples R China
[2] Tongji Univ, Coll Environm Sci & Engn, State Key Lab Pollut Control & Resource Reuse, Shanghai 200092, Peoples R China
基金
中国国家自然科学基金;
关键词
Struvite; Nutrient recovery; Zn(II) sorption; Zinc immobilization; Waste recycling; HEAVY-METALS; IMMOBILIZATION; ADSORPTION; EXTRACTION; ZN; PB; CU;
D O I
10.1007/s10311-017-0694-3
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Zinc is known as an essential element of human life. However, excessive zinc discharge into water and soil causes water pollution, leading to serious health issues such as septicemia, meningitis and iron-deficiency anemia. Here, a novel material made of struvite-supported diatomite was obtained from eutrophic water treated by mesoporous MgO-modified diatomite. This material was applied for zinc remediation in aqueous solutions and contaminated soils to test the reuse of P-containing products. Struvite-supported diatomite was characterized by field emission scanning electron microscopy and X-ray diffraction. Results show that the maximum removal efficiency of Zn(II) from wastewater streams reached 90.54% at an initial pH of 5 and struvite-supported diatomite dosage of 0.3 g/L. Moreover, the X-ray diffraction patterns of precipitates after Zn(II) sorption show that the combination between zinc and the phosphate group played a key role for zinc removal in solution. For Zn-contaminated soils amended with 10% struvite-supported diatomite, available Zn decreased by 65.38% and acid soluble Zn decreased by 56.9% after 56 days.
引用
收藏
页码:569 / 573
页数:5
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