Synthesis of g-C3N4 with heating acetic acid treated melamine and its photocatalytic activity for hydrogen evolution

被引:125
作者
Wu, Ming [1 ]
Yan, Jun-Min [1 ]
Zhang, Xue-wei [1 ]
Zhao, Ming [1 ]
机构
[1] Jilin Univ, Dept Mat Sci & Engn, Key Lab Automobile Mat, Minist Educ, Renming St, Changchun 130022, Peoples R China
基金
中国国家自然科学基金;
关键词
g-C3N4; Photocatalyst; Hydrogen; Visible light; GRAPHITIC CARBON NITRIDE; SEMICONDUCTORS; WATER; HETEROJUNCTION; NANOSHEETS; CATALYSIS;
D O I
10.1016/j.apsusc.2015.01.132
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The g-C3N4 is synthesized by directly heating the acetic acid treatment melamine. A combination of XRD, SEM, TEM, PL and UV-vis are utilized to characterize the composition, morphology and optical properties of g-C3N4. This method synthesized g-C3N4 shows smaller particles and some holes which high up the photocatalytic activity compared with the bulk g-C3N4. 2015 Elsevier B.V. All rights reserved.
引用
收藏
页码:196 / 200
页数:5
相关论文
共 47 条
  • [1] Ionothermal Synthesis of Crystalline, Condensed, Graphitic Carbon Nitride
    Bojdys, Michael J.
    Mueller, Jens-Oliver
    Antonietti, Markus
    Thomas, Arne
    [J]. CHEMISTRY-A EUROPEAN JOURNAL, 2008, 14 (27) : 8177 - 8182
  • [2] Graphitic carbon nitride (g-C3N4)-Pt-TiO2 nanocomposite as an efficient photocatalyst for hydrogen production under visible light irradiation
    Chai, Bo
    Peng, Tianyou
    Mao, Jing
    Li, Kan
    Zan, Ling
    [J]. PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2012, 14 (48) : 16745 - 16752
  • [3] Titanium dioxide nanomaterials: Synthesis, properties, modifications, and applications
    Chen, Xiaobo
    Mao, Samuel S.
    [J]. CHEMICAL REVIEWS, 2007, 107 (07) : 2891 - 2959
  • [4] Increasing Solar Absorption for Photocatalysis with Black Hydrogenated Titanium Dioxide Nanocrystals
    Chen, Xiaobo
    Liu, Lei
    Yu, Peter Y.
    Mao, Samuel S.
    [J]. SCIENCE, 2011, 331 (6018) : 746 - 750
  • [5] Fe-g-C3N4-Catalyzed Oxidation of Benzene to Phenol Using Hydrogen Peroxide and Visible Light
    Chen, Xiufang
    Zhang, Jinshui
    Fu, Xianzhi
    Antonietti, Markus
    Wang, Xinchen
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2009, 131 (33) : 11658 - +
  • [6] Band Structure Engineering of Carbon Nitride: In Search of a Polymer Photocatalyst with High Photooxidation Property
    Chu, Sheng
    Wang, Ying
    Guo, Yong
    Feng, Jianyong
    Wang, Cuicui
    Luo, Wenjun
    Fan, Xiaoxing
    Zou, Zhigang
    [J]. ACS CATALYSIS, 2013, 3 (05): : 912 - 919
  • [7] Construction of Conjugated Carbon Nitride Nanoarchitectures in Solution at Low Temperatures for Photoredox Catalysis
    Cui, Yanjuan
    Ding, Zhengxin
    Fu, Xianzhi
    Wang, Xinchen
    [J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2012, 51 (47) : 11814 - 11818
  • [8] ELECTROCHEMICAL PHOTOLYSIS OF WATER AT A SEMICONDUCTOR ELECTRODE
    FUJISHIMA, A
    HONDA, K
    [J]. NATURE, 1972, 238 (5358) : 37 - +
  • [9] Synthesis and characterization of composite visible light active photocatalysts MoS2-g-C3N4 with enhanced hydrogen evolution activity
    Ge, Lei
    Han, Changcun
    Xiao, Xinlai
    Guo, Lele
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2013, 38 (17) : 6960 - 6969
  • [10] Synthesis and Efficient Visible Light Photocatalytic Hydrogen Evolution of Polymeric g-C3N4 Coupled with CdS Quantum Dots
    Ge, Lei
    Zuo, Fan
    Liu, Jikai
    Ma, Quan
    Wang, Chen
    Sun, Dezheng
    Bartels, Ludwig
    Feng, Pingyun
    [J]. JOURNAL OF PHYSICAL CHEMISTRY C, 2012, 116 (25) : 13708 - 13714