Multidimensional spectroscopy with a single broadband phase-shaped laser pulse

被引：5

作者：

Glenn, Rachel ^{[1
]}

Mukamel, Shaul ^{[1
]}

机构：

[1] Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA

来源：

JOURNAL OF CHEMICAL PHYSICS | 2014年 / 140卷 / 14期

基金：

美国国家科学基金会;

关键词：

COHERENT CONTROL; FEMTOSECOND; DYNAMICS;

D O I：

10.1063/1.4869750

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

We calculate the frequency-dispersed nonlinear transmission signal of a phase-shaped visible pulse to fourth order in the field. Two phase profiles, a phase-step and phase-pulse, are considered. Two dimensional signals obtained by varying the detected frequency and phase parameters are presented for a three electronic band model system. We demonstrate how two-photon and stimulated Raman resonances can be manipulated by the phase profile and sign, and selected quantum pathways can be suppressed. (C) 2014 AIP Publishing LLC.

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页数：13

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