Co atoms on Bi2Se3 revealing a coverage dependent spin reorientation transition

被引:17
作者
Eelbo, T. [1 ]
Sikora, M. [2 ]
Bihlmayer, G. [3 ,4 ,5 ]
Dobrzanski, M. [2 ]
Kozlowski, A. [2 ]
Miotkowski, I. [6 ]
Wiesendanger, R. [1 ]
机构
[1] Univ Hamburg, Inst Appl Phys, D-20355 Hamburg, Germany
[2] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland
[3] Forschungszentrum Julich, Peter Grunberg Inst, D-52428 Julich, Germany
[4] Forschungszentrum Julich, Inst Adv Simulat, D-52428 Julich, Germany
[5] JARA, D-52428 Julich, Germany
[6] Purdue Univ, Dept Phys, W Lafayette, IN 47907 USA
来源
NEW JOURNAL OF PHYSICS | 2013年 / 15卷
关键词
SURFACE; ANISOTROPY;
D O I
10.1088/1367-2630/15/11/113026
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We investigate Co nanostructures on Bi2Se3 by means of scanning tunneling microscopy and spectroscopy (STM/STS), x-ray absorption spectroscopy, x-ray magnetic dichroism (XMCD) and calculations using the density functional theory (DFT). In the single adatom regime we find two different adsorption sites by STM. Our calculations reveal these to be the fcc and hcp hollow sites of the substrate. STS shows a pronounced peak for only one species of the Co adatoms indicating different electronic properties of both types. These are explained on the basis of our DFT calculations by different hybridizations with the substrate. Using XMCD we find a coverage dependent spin reorientation transition from easy-plane toward out-of-plane. We suggest clustering to be the predominant cause for this observation.
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页数:10
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共 26 条
  • [1] Coexistence of the topological state and a two-dimensional electron gas on the surface of Bi2Se3
    Bianchi, Marco
    Guan, Dandan
    Bao, Shining
    Mi, Jianli
    Iversen, Bo Brummerstedt
    King, Philip D. C.
    Hofmann, Philip
    [J]. NATURE COMMUNICATIONS, 2010, 1
  • [2] Magnetocrystalline anisotropy energy of Co and Fe adatoms on the (111) surfaces of Pd and Rh
    Blonski, Piotr
    Lehnert, Anne
    Dennler, Samuel
    Rusponi, Stefano
    Etzkorn, Markus
    Moulas, Geraud
    Bencok, Peter
    Gambardella, Pietro
    Brune, Harald
    Hafner, Juergen
    [J]. PHYSICAL REVIEW B, 2010, 81 (10)
  • [3] TIGHT-BINDING APPROACH TO THE ORBITAL MAGNETIC-MOMENT AND MAGNETOCRYSTALLINE ANISOTROPY OF TRANSITION-METAL MONOLAYERS
    BRUNO, P
    [J]. PHYSICAL REVIEW B, 1989, 39 (01): : 865 - 868
  • [4] Experimental Observation of the Quantum Anomalous Hall Effect in a Magnetic Topological Insulator
    Chang, Cui-Zu
    Zhang, Jinsong
    Feng, Xiao
    Shen, Jie
    Zhang, Zuocheng
    Guo, Minghua
    Li, Kang
    Ou, Yunbo
    Wei, Pang
    Wang, Li-Li
    Ji, Zhong-Qing
    Feng, Yang
    Ji, Shuaihua
    Chen, Xi
    Jia, Jinfeng
    Dai, Xi
    Fang, Zhong
    Zhang, Shou-Cheng
    He, Ke
    Wang, Yayu
    Lu, Li
    Ma, Xu-Cun
    Xue, Qi-Kun
    [J]. SCIENCE, 2013, 340 (6129) : 167 - 170
  • [5] EXPERIMENTAL CONFIRMATION OF THE X-RAY MAGNETIC CIRCULAR-DICHROISM SUM-RULES FOR IRON AND COBALT
    CHEN, CT
    IDZERDA, YU
    LIN, HJ
    SMITH, NV
    MEIGS, G
    CHABAN, E
    HO, GH
    PELLEGRIN, E
    SETTE, F
    [J]. PHYSICAL REVIEW LETTERS, 1995, 75 (01) : 152 - 155
  • [6] Massive Dirac Fermion on the Surface of a Magnetically Doped Topological Insulator
    Chen, Y. L.
    Chu, J. -H.
    Analytis, J. G.
    Liu, Z. K.
    Igarashi, K.
    Kuo, H. -H.
    Qi, X. L.
    Mo, S. K.
    Moore, R. G.
    Lu, D. H.
    Hashimoto, M.
    Sasagawa, T.
    Zhang, S. C.
    Fisher, I. R.
    Hussain, Z.
    Shen, Z. X.
    [J]. SCIENCE, 2010, 329 (5992) : 659 - 662
  • [7] Topological insulators in three dimensions
    Fu, Liang
    Kane, C. L.
    Mele, E. J.
    [J]. PHYSICAL REVIEW LETTERS, 2007, 98 (10)
  • [8] Giant magnetic anisotropy of single cobalt atoms and nanoparticles
    Gambardella, P
    Rusponi, S
    Veronese, M
    Dhesi, SS
    Grazioli, C
    Dallmeyer, A
    Cabria, I
    Zeller, R
    Dederichs, PH
    Kern, K
    Carbone, C
    Brune, H
    [J]. SCIENCE, 2003, 300 (5622) : 1130 - 1133
  • [9] Localized magnetic states of Fe, Co, and Ni impurities on alkali metal films
    Gambardella, P
    Dhesi, SS
    Gardonio, S
    Grazioli, C
    Ohresser, P
    Carbone, C
    [J]. PHYSICAL REVIEW LETTERS, 2002, 88 (04) : 4 - 472024
  • [10] In-Plane Magnetic Anisotropy of Fe Atoms on Bi2Se3(111)
    Honolka, J.
    Khajetoorians, A. A.
    Sessi, V.
    Wehling, T. O.
    Stepanow, S.
    Mi, J. -L.
    Iversen, B. B.
    Schlenk, T.
    Wiebe, J.
    Brookes, N. B.
    Lichtenstein, A. I.
    Hofmann, Ph.
    Kern, K.
    Wiesendanger, R.
    [J]. PHYSICAL REVIEW LETTERS, 2012, 108 (25)