Active Liquid Crystal Tuning of Metallic Nanoantenna Enhanced Light Emission from Colloidal Quantum Dots

被引:47
作者
Abass, Aimi [1 ]
Rodriguez, Said Rahimzadeh-Kalaleh [2 ]
Ako, Thomas [3 ]
Aubert, Tangi [4 ,5 ]
Verschuuren, Marc [6 ]
Van Thourhout, Dries [5 ,7 ]
Beeckman, Jeroen [3 ,5 ]
Hens, Zeger [4 ,5 ]
Rivas, Jaime Gomez [2 ,8 ]
Maes, Bjorn [7 ,9 ]
机构
[1] Univ Ghent, Dept Elect & Informat Syst ELIS, Solar Cells Grp, B-9000 Ghent, Belgium
[2] FOM Inst AMOLF, Ctr Nanophoton, Philips Res Labs, NL-5656 AE Eindhoven, Netherlands
[3] Univ Ghent, Dept Elect & Informat Syst ELIS, Liquid Crystals & Photon Grp, B-9000 Ghent, Belgium
[4] Univ Ghent, Dept Inorgan & Phys Chem, Phys & Chem Nanostruct, B-9000 Ghent, Belgium
[5] Univ Ghent, Ctr Nano & Biophoton NB Photon, B-9000 Ghent, Belgium
[6] Philips Res Labs, NL-5656 AE Eindhoven, Netherlands
[7] Univ Ghent, IMEC, Photon Res Grp INTEC, B-9000 Ghent, Belgium
[8] Eindhoven Univ Technol, COBRA Res Inst, NL-5600 MB Eindhoven, Netherlands
[9] Univ Mons, Fac Sci, Micro & Nanophoton Mat Grp, B-7000 Mons, Belgium
关键词
Waveguide; nanoantenna; liquid crystal; quantum dot; fluorescence; SURFACE-PLASMON RESONANCE; DIRECTIONAL EMISSION; REFRACTIVE-INDEXES; LINE-SHAPES; NANOPARTICLES; ARRAYS; DISPERSION; SCATTERING;
D O I
10.1021/nl501955e
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A system comprising an aluminum nanoantenna array on top of a luminescent colloidal quantum dot waveguide and covered by a thermotropic liquid crystal (LC) is introduced. By heating the LC above its critical temperature, we demonstrate that the concomitant refractive index change modifies the hybrid plasmonic-photonic resonances in the system. This enables active control of the spectrum and directionality of the narrow-band (similar to 6 nm) enhancement of quantum dot photoluminescence by the metallic nanoantennas.
引用
收藏
页码:5555 / 5560
页数:6
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