ZnCr-LDH/N-doped graphitic carbon-incorporated g-C 3 N 4 2D/2D nanosheet heterojunction with enhanced charge transfer for photocatalysis

被引：62
作者：
Liu, Jun [1 ]
Li, Jia [1 ]
Bing, Xingmei [1 ]
Ng, Dickon H. L. [2 ]
Cui, Xinling [1 ]
Ji, Fei [1 ]
Kionga, Denis Dienguila [1 ]
机构：
[1] Univ Jinan, Sch Mat Sci & Engn, Jinan, Shandong, Peoples R China
[2] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China
来源：
MATERIALS RESEARCH BULLETIN | 2018年 / 102卷
基金：
中国国家自然科学基金;
关键词：
g-C(3)N4; ZnCr-LDH; 2D-2D; Heterogeneous; Photocatalyst; LAYERED DOUBLE HYDROXIDE; MAGNETIC MICROSPHERES; HYDROGEN-PRODUCTION; FACILE SYNTHESIS; RHODAMINE-B; G-C3N4; ADSORPTION; NITRIDE; REMOVAL; ROUTE;
D O I：
10.1016/j.materresbull.2018.03.010
中图分类号：
T [工业技术];
学科分类号：
08 ;
摘要：
In this work, we successfully synthesized a novel ZnCr-LDH/N-doped graphitic carbon-incorporated g-C3N4 (g-C3N4-C(N)) hybrid with unique two-dimensional/two-dimensional (2D-2D) structure for the efficient degradation of Congo red under visible light irradiation. It was demonstrated that ZnCr-LDH/g-C3N4-C(N) exhibited lower photogenerated electron-hole recombination rate and enhanced light harvesting. Furthermore, its derived calcined product also showed outstanding performance due to the unique heterogeneous structure and the synergistic effect between photocatalysis and adsorption. In addition, the mixed metal oxide ZnO and ZnCr2O4 in ZnCr-CLDH/g-C3N4-C(N) dispersed uniformly on the g-C3N4-C(N) exposed more active sites and facilitated the photodegradation of pollutants.
引用
收藏
页码：379 / 390
页数：12
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