Trends in Solid Adsorbent Materials Development for CO2 Capture

被引:280
作者
Pardakhti, Maryam [1 ]
Jafari, Tahereh [2 ]
Tobin, Zachary [3 ]
Dutta, Biswanath [3 ]
Moharreri, Ehsan [2 ]
Shemshaki, Nikoo S. [4 ]
Suib, Steven [2 ,3 ]
Srivastava, Ranjan [1 ]
机构
[1] Univ Connecticut, Dept Chem & Biomol Engn, Storrs, CT 06269 USA
[2] Univ Connecticut, Inst Mat Sci, Storrs, CT 06269 USA
[3] Univ Connecticut, Dept Chem, Storrs, CT 06269 USA
[4] Univ Connecticut, Dept Biomed Engn, Storrs, CT 06269 USA
关键词
CO2 adsorption and separation; carbon capture; porous materials; solid adsorbent; surface functionalization; METAL-ORGANIC-FRAMEWORKS; CARBON-DIOXIDE CAPTURE; DENSITY-FUNCTIONAL THEORY; TRIAZINE-BASED FRAMEWORKS; MOLECULAR-DYNAMICS SIMULATIONS; HIGH-SURFACE-AREA; N-DOPED CARBON; ACTIVATED CARBON; GAS-ADSORPTION; COORDINATION POLYMERS;
D O I
10.1021/acsami.9b08487
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
A recent report from the United Nations has warned about the excessive CO2 emissions and the necessity of making efforts to keep the increase in global temperature below 2 degrees C. Current CO2 capture technologies are inadequate for reaching that goal, and effective mitigation strategies must be pursued. In this work, we summarize trends in materials development for CO2 adsorption with focus on recent studies. We put adsorbent materials into four main groups: (I) carbon-based materials, (II) silica/alumina/zeolites, (III) porous crystalline solids, and (IV) metal oxides. Trends in computational investigations along with experimental findings are covered to find promising candidates in light of practical challenges imposed by process economics.
引用
收藏
页码:34533 / 34559
页数:27
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