High-Rate Oxygen Evolution Reaction on Al-Doped LiNiO2

被引：87

作者：

Gupta, Asha ^{[1
]}

Chemelewski, William D. ^{[1
]}

Mullins, C. Buddie ^{[1
,2
,3
]}

Goodenough, John B. ^{[1
]}

机构：

[1] Univ Texas Austin, Texas Mat Inst, Austin, TX 78712 USA

[2] Univ Texas Austin, McKetta Dept Chem Engn, Austin, TX 78712 USA

[3] Univ Texas Austin, Dept Chem, Austin, TX 78712 USA

来源：

ADVANCED MATERIALS | 2015年 / 27卷 / 39期

关键词：

Al-doped LiNiO2; electrocatalysis; oxygen evolution reaction; solution combustion synthesis; X-ray photoelectron spectroscopy (XPS); ELECTROCHEMICAL PROPERTIES; WATER OXIDATION; ALKALINE MEDIA; OXIDE; REDUCTION; BATTERIES; CATALYSTS; NANOSTRUCTURES; EFFICIENT; ALUMINUM;

D O I：

10.1002/adma.201502256

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

LiNi0.8Al0.2O2 with a higher Ni3+/Li+ ordering, synthesized by the solution-combustion method, gives oxygen-evolution-reaction (OER) activity in alkaline solution that is comparable to that of IrO2. This confirms that the octahedral-site Ni-IV/Ni-III couple in an oxide is an active redox center for the OER with redox energy pinned at the top of the O-2p bands.

引用

页码：6063 / 6067

页数：5

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