Angle-resolved photoemission spectroscopy and magnetic circular dichroism in Fe-intercalated TiS2

被引:16
|
作者
Yamasaki, A [1 ]
Imada, S
Sekiyama, A
Suga, S
Matsushita, T
Muro, T
Saitoh, Y
Negishi, H
Sasaki, M
机构
[1] Osaka Univ, Grad Sch Engn Sci, Div Mat Phys, Osaka 5608531, Japan
[2] Japan Synchrotron Radiat Res Inst, Mikazuki, Hyogo 6795148, Japan
[3] Japan Atom Energy Res Inst, Mikazuki, Hyogo 6795148, Japan
[4] Hiroshima Univ, Grad Sch Adv Sci Matter, Higashihiroshima 7398526, Japan
关键词
D O I
10.1142/S0218625X02003160
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
In order to directly investigate the energy band dispersion and the origin of the magnetic moment in intercalation compounds FexTiS2, we have measured the angle-resolved photoemission (ARPES) spectrum and the magnetic circular dichroism (MCD) of the soft X-ray core absorption (XAS) spectra using a synchrotron light source. The energy band dispersion is clearly observed in the Ti 2p(3/2)(e(g)) on-resonance ARPES spectra. In the Ti 2p XAS spectra the MCD is clearly seen, suggesting that a magnetic moment is induced on the Ti atom through the hybridization with the Fe 3d orbitals. We quantitatively estimate the orbital and spin magnetic moments of the Fe and Ti atoms by using the magneto-optical sum rules.
引用
收藏
页码:961 / 966
页数:6
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