Radon volumetric activity and ion production in the undisturbed lower atmosphere: Ground-based observations and numerical modeling

The results of in situ ground-based observations of radon volumetric activity carried out at the Borok Geophysical Observatory of Schmidt Institute of Physics of the Earth of the Russian Academy of Sciences (58A degrees 04' N; 38A degrees 14' E) are presented. Modeling the characteristic diurnal variation in the ion production rate in the undisturbed midlatitude lower atmosphere above land is carried out. The Lagrangian stochastic model of turbulent transport is developed in application to determining the vertical profiles of radon activity for 222Rn and 220Rn isotopes and their radioactive decay products. The results calculated by the Lagrangian stochastic model are matched with the analytical solution for the free atmosphere. Based on the model, the estimate is obtained for the rate of radon outflow from the convective boundary layer to the free clear sky atmosphere. The implications of temperature stratification of the atmosphere for the vertical distribution of the ion production rate at the different radon emission rate are explored.