Emergence of quasiparticles in a doped Mott insulator

被引:11
|
作者
Wang, Yao [1 ]
He, Yu [2 ,3 ,4 ]
Wohlfeld, Krzysztof [5 ]
Hashimoto, Makoto [6 ]
Huang, Edwin W. [3 ,4 ,7 ,8 ,9 ,10 ]
Lu, Donghui [6 ]
Mo, Sung-Kwan [11 ]
Komiya, Seiki [12 ]
Jia, Chunjing [3 ,4 ]
Moritz, Brian [3 ,4 ]
Shen, Zhi-Xun [3 ,4 ,7 ,8 ]
Devereaux, Thomas P. [3 ,4 ,13 ]
机构
[1] Clemson Univ, Dept Phys & Astron, Clemson, SC 29631 USA
[2] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA
[3] SLAC Natl Accelerator Lab, Stanford Inst Mat & Energy Sci, Menlo Pk, CA 94025 USA
[4] Stanford Univ, Menlo Pk, CA 94025 USA
[5] Univ Warsaw, Fac Phys, Inst Theoret Phys, Pasteura 5, PL-02093 Warsaw, Poland
[6] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA
[7] Stanford Univ, Dept Phys, Stanford, CA 94305 USA
[8] Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA
[9] Univ Illinois, Dept Phys, Urbana, IL 61801 USA
[10] Univ Illinois, Inst Condensed Matter Theory, Urbana, IL 61801 USA
[11] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA
[12] Cent Res Inst Elect Power Ind, Yokosuka, Kanagawa 2400196, Japan
[13] Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA
基金
美国国家科学基金会;
关键词
SPECTRAL WEIGHT; FERMI-SURFACE; TEMPERATURE; SUPERCONDUCTIVITY; CHARGE; EXCITATIONS; DYNAMICS; ENERGY; OXYGEN; STATES;
D O I
10.1038/s42005-020-00480-5
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The emergence of quasiparticles in a doped Mott insulator is the key to understanding high Tc cuprate superconductivity - a major quest in condensed matter physics. Here, the authors investigate the angle-resolved photoemission spectroscopy in the cuprates and observe how the quasiparticle emerges from the Mott insulating regime. How a Mott insulator develops into a weakly coupled metal upon doping is a central question to understanding various emergent correlated phenomena. To analyze this evolution and its connection to the high-T-c cuprates, we study the single-particle spectrum for the doped Hubbard model using cluster perturbation theory on superclusters. Starting from extremely low doping, we identify a heavily renormalized quasiparticle dispersion that immediately develops across the Fermi level, and a weakening polaronic side band at higher binding energy. The quasiparticle spectral weight roughly grows at twice the rate of doping in the low doping regime, but this rate is halved at optimal doping. In the heavily doped regime, we find both strong electron-hole asymmetry and a persistent presence of Mott spectral features. Finally, we discuss the applicability of the single-band Hubbard model to describe the evolution of nodal spectra measured by angle-resolved photoemission spectroscopy (ARPES) on the single-layer cuprate La2-xSrxCuO4 (0 <= x <= 0.15). This work benchmarks the predictive power of the Hubbard model for electronic properties of high-T-c cuprates.
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页数:7
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