Phase-field-crystal modeling of glass-forming liquids: Spanning time scales during vitrification, aging, and deformation

被引:16
|
作者
Berry, Joel [1 ]
Grant, Martin [1 ]
机构
[1] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada
来源
PHYSICAL REVIEW E | 2014年 / 89卷 / 06期
关键词
DENSITY-FUNCTIONAL THEORY; COUPLING THEORY; DYNAMICS; TRANSITION;
D O I
10.1103/PhysRevE.89.062303
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
Two essential elements required to generate a glass transition within phase-field-crystal (PFC) models are outlined based on observed freezing behaviors in various models of this class. The central dynamic features of glass formation in simple binary liquids are qualitatively reproduced across 12 orders of magnitude in time by applying a physically motivated time scaling to previous PFC simulation results. New aspects of the equilibrium phase behavior of the same binary model system are also outlined, aging behavior is explored in the moderate and deeply supercooled regimes, and aging exponents are extracted. General features of the elastic and plastic responses of amorphous and crystalline PFC solids under deformation are also compared and contrasted.
引用
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页数:10
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