Leaching is a complex solid-liquid reaction which has an important influence on the recovery efficiency of the spent lithium-ion batteries (LIBs). Therefore, it is of significant importance to utilize an appropriate technique to predict the effect of operating parameters on the optimized recovery rate. In the present study, a combined method of the artificial neural network (ANN) and particle swarm optimization algorithm (PSO) was used as a model to predict the leaching efficiency of cobalt from spent LIBs. To find the dependency of the leached percentage of cobalt on the operational parameters as model inputs, 42 repeatable numerous experiments are performed using H2SO4 in the presence of H2O2. It was found that the proposed model can be a useful technique in the demonstration of the nonlinear relationship between the leaching efficiency and the process parameters. The performance of PSO-ANN models was validated by statistical thresholds and compared with those of common ANN technique. Moreover, it was found that the pulp density of the leaching solution and the concentration of sulfuric acid were the most important reaction parameters of the spent LIBs recovery, respectively.
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Univ Tokyo, Fac Engn, Dept Chem Syst Engn, Bunkyo Ku, Tokyo 1138656, JapanTohoku Univ, Res Ctr Sustainable Sci & Engn, Inst Multidisciplinary Res Adv Mat, Sendai, Miyagi 9808577, Japan
Yamashita, Yasunobu
Nagasawa, Hiroki
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Univ Tokyo, Grad Sch Frontier Sci, Dept Environm Syst, Chiba 2778563, JapanTohoku Univ, Res Ctr Sustainable Sci & Engn, Inst Multidisciplinary Res Adv Mat, Sendai, Miyagi 9808577, Japan
Nagasawa, Hiroki
Yamasaki, Akihiro
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Seikei Univ, Fac Sci & Technol, Dept Mat & Life Sci, Musashino, Tokyo 1808633, JapanTohoku Univ, Res Ctr Sustainable Sci & Engn, Inst Multidisciplinary Res Adv Mat, Sendai, Miyagi 9808577, Japan
Yamasaki, Akihiro
Yanagisawa, Yukio
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Univ Tokyo, Grad Sch Frontier Sci, Dept Environm Syst, Chiba 2778563, JapanTohoku Univ, Res Ctr Sustainable Sci & Engn, Inst Multidisciplinary Res Adv Mat, Sendai, Miyagi 9808577, Japan
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Univ New South Wales, Ctr Sustainable Mat Res & Technol SMaRT, Sch Mat Sci & Engn, Sydney, NSW 2052, AustraliaUniv New South Wales, Ctr Sustainable Mat Res & Technol SMaRT, Sch Mat Sci & Engn, Sydney, NSW 2052, Australia
Maroufi, Samane
Assefi, Mohammad
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Univ New South Wales, Ctr Sustainable Mat Res & Technol SMaRT, Sch Mat Sci & Engn, Sydney, NSW 2052, AustraliaUniv New South Wales, Ctr Sustainable Mat Res & Technol SMaRT, Sch Mat Sci & Engn, Sydney, NSW 2052, Australia
Assefi, Mohammad
Nekouei, Rasoul Khayyam
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Univ New South Wales, Ctr Sustainable Mat Res & Technol SMaRT, Sch Mat Sci & Engn, Sydney, NSW 2052, AustraliaUniv New South Wales, Ctr Sustainable Mat Res & Technol SMaRT, Sch Mat Sci & Engn, Sydney, NSW 2052, Australia
Nekouei, Rasoul Khayyam
Sahajwalla, Veena
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Univ New South Wales, Ctr Sustainable Mat Res & Technol SMaRT, Sch Mat Sci & Engn, Sydney, NSW 2052, AustraliaUniv New South Wales, Ctr Sustainable Mat Res & Technol SMaRT, Sch Mat Sci & Engn, Sydney, NSW 2052, Australia
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Korea Inst Geosci & Mineral Resources KIGAM, Resources Utilizat Res Div, Daejeon, South KoreaKorea Inst Geosci & Mineral Resources KIGAM, Resources Utilizat Res Div, Daejeon, South Korea
Shim, Hyun-woo
Im, Byoungyong
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Inst Adv Engn IAE, Mat Sci & Chem Engn Ctr, 51 Goan Rd, Gyeonggi 17180, Yongin, South Korea
Sejong Univ, Dept Nanotechnol & Adv Mat Engn, Seoul, South KoreaKorea Inst Geosci & Mineral Resources KIGAM, Resources Utilizat Res Div, Daejeon, South Korea
Im, Byoungyong
Joo, Soyeong
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Inst Adv Engn IAE, Mat Sci & Chem Engn Ctr, 51 Goan Rd, Gyeonggi 17180, Yongin, South KoreaKorea Inst Geosci & Mineral Resources KIGAM, Resources Utilizat Res Div, Daejeon, South Korea
Joo, Soyeong
Kim, Dae-guen
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Inst Adv Engn IAE, Mat Sci & Chem Engn Ctr, 51 Goan Rd, Gyeonggi 17180, Yongin, South KoreaKorea Inst Geosci & Mineral Resources KIGAM, Resources Utilizat Res Div, Daejeon, South Korea