Measurement of 100Mo(n, 2n)99Mo reaction cross-sections using 10-20 MeV quasi-monoenergetic neutrons

被引:0
作者
Parashari, Siddharth [1 ]
Mukherjee, Surjit [1 ]
Makwana, Rajnikant [1 ]
Singh, N. L. [1 ]
Singh, Ratan K. [1 ]
Naik, H. [2 ]
Suryanarayana, S., V [3 ]
Nayak, B. K. [3 ]
Sharma, S. C. [3 ]
Mehta, Mayur [4 ]
Ayyala, Sai Akhil [5 ]
Varmuza, Jan [6 ]
Katovsky, Karel [6 ]
机构
[1] MS Univ, Dept Phys, Vadodara, India
[2] Bhabha Atom Res Ctr, Radiochem Div, Bombay, Maharashtra, India
[3] Bhabha Atom Res Ctr, Nucl Phys Div, Bombay, Maharashtra, India
[4] Inst Plasma Res, Gandhinagar, India
[5] GB Pant Univ Ag & Tech, Uttarakhand, India
[6] Brno Univ Technol, Dept Elect Power Engn, Brno, Czech Republic
来源
PROCEEDINGS OF THE 2018 19TH INTERNATIONAL SCIENTIFIC CONFERENCE ON ELECTRIC POWER ENGINEERING (EPE) | 2018年
关键词
Mo-100(n; 2n); reaction; Li-7(p; n) reaction for neutrons; cross section; gamma-rayspectroscopy; ALICE; TALYS; calculation; NUCLEAR-DATA LIBRARY; EXCITATION-FUNCTIONS; ISOTOPES; MOLYBDENUM; TC-99M; EXFOR; MO-99;
D O I
10.1109/EPE.2018.8395960
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
The production cross-sections for the medical isotope Mo-99 were measured using Mo-100(n, 2n) reaction at average neutron energies of 10.95 +/- 0.45, 13.97 +/- 0.68, 16.99 +/- 0.53 and 20.00 +/- 0.58 MeV using the off-line gamma-ray spectroscopy. The neutrons of desired energies were generated using Li-7 (p, n) reaction at 14UD BARC-TIFR Pelletron facility, Mumbai, India. The experimentally measured data from the present work have been compared with the existing data libraries like, ENDF/B-VII.1, JENDL-4.0, JEFF-3.2 and CENDL-3.1. The results were also reproduced and compared with the theoretical nuclear modular codes like TALYS-1.8, and ALICE-2014. A modified set of parameters is also used to fit the existing data more accurately. The present findings show a good agreement with the theoretical as well as with the existing experimental data in different data libraries.
引用
收藏
页数:5
相关论文
共 50 条
[21]   Cross-sections of 45Sc(n, 2n)44m,gSc reaction from the reaction threshold to 20 MeV [J].
Luo, J. ;
Liu, R. ;
Jiang, L. ;
Liu, Z. ;
Sun, G. ;
Ge, S. .
RADIOCHIMICA ACTA, 2013, 101 (10) :607-612
[22]   Measurement of the (n, 2n) reaction cross-sections of iodine and cesium induced by D-T neutrons with covariance analysis* [J].
Lan, Changlin ;
Niu, Yuxing ;
Wei, Yuting ;
Lu, Fangxiao ;
Yang, Xianlin ;
Xu, Ruirui ;
Zhang, Yue ;
Ge, Yujie ;
Wang, Jiahao ;
Jiang, Gong .
CHINESE PHYSICS C, 2023, 47 (09)
[23]   Measurements of the thermal neutron cross-sections and resonance integrals for 186W (n,γ) 187W and 98Mo (n,γ) 99Mo reactions [J].
A. El Abd .
Journal of Radioanalytical and Nuclear Chemistry, 2010, 284 :321-326
[24]   Evaluation of excitation functions of 100Mo(p,d+pn)99Mo and 100Mo (p,2n)99mTc reactions: Estimation of long-lived Tc-impurity and its implication on the specific activity of cyclotron-produced 99mTc [J].
Qaim, S. M. ;
Sudar, S. ;
Scholten, B. ;
Koning, A. J. ;
Coenen, H. H. .
APPLIED RADIATION AND ISOTOPES, 2014, 85 :101-113
[25]   Measurement of 232Th(n,2n)231Th reaction cross-sections at neutron energies of 14.1 MeV and 14.8 MeV using neutron activation method [J].
Lan Chang-Lin ;
Xie Bao-Lin ;
Zhang Kai ;
Peng Meng ;
Fang Kai-Hong .
NUCLEAR SCIENCE AND TECHNIQUES, 2015, 26 (06)
[26]   Determination of the experimental yield of 99mTc in (p,2n) nuclear reaction on enriched 100Mo sample with application of 11-MeV medical cyclotron [J].
Bondar, B. M. ;
Leshchenko, B. Yu. ;
Kadenko, I. M. ;
Kmetyuk, Ya. V. .
APPLIED RADIATION AND ISOTOPES, 2022, 189
[27]   Neural network predictions of (n,2n) reaction cross-sections at 14.6 MeV incident neutron energy [J].
Akkoyun, Serkan ;
Amrani, Naima ;
Bayram, Tuncay .
APPLIED RADIATION AND ISOTOPES, 2023, 191
[28]   Activation cross section measurement of the 100Mo(α,n)103Ru reaction for optical potential studies [J].
Szegedi, T. N. ;
Kiss, G. G. ;
Gyurky, Gy ;
Mohr, P. .
NUCLEAR PHYSICS IN ASTROPHYSICS IX (NPA-IX), 2020, 1668
[29]   (n, 2n), (n, p) and (n, α) Reactions cross-sections measurement on selenium isotopes at neutron energy of 14MeV [J].
He Guo-Zhu ;
Tuo Fei ;
Kong Xiang-Zhong .
HIGH ENERGY PHYSICS AND NUCLEAR PHYSICS-CHINESE EDITION, 2006, 30 (09) :844-847
[30]   Selection of key parameters for the high yield production of 99mTc via 100Mo (p, 2n) 99mTc reaction in a cyclotron [J].
Yu, Yue ;
Chen, Zhi .
RADIATION PHYSICS AND CHEMISTRY, 2025, 232