Probing excitons and biexcitons in coupled quantum dots by coherent two-dimensional optical spectroscopy

被引:7
作者
Kavousanaki, E. G. [1 ]
Roslyak, O. [1 ]
Mukamel, S. [1 ]
机构
[1] Univ Calif Irvine, Dept Chem, Irvine, CA 92617 USA
来源
PHYSICAL REVIEW B | 2009年 / 79卷 / 15期
基金
美国国家科学基金会;
关键词
biexcitons; gallium arsenide; hopping conduction; III-V semiconductors; indium compounds; infrared spectra; photon echo; semiconductor quantum dots; ultraviolet spectra; visible spectra; SEMICONDUCTOR NANOCRYSTALS; SYSTEMS; INFORMATION;
D O I
10.1103/PhysRevB.79.155324
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We calculate two-dimensional (2D) photon-echo and double-quantum-coherence spectra of two coupled InGaAs/GaAs quantum dots at various distances, taking into account electron, hole, and exciton hopping. Signatures of direct and indirect excitons in two-exciton resonances are revealed. At short distances, electron delocalization contributes to the creation of new biexcitonic peaks, and dipole-dipole interactions shift the two-exciton energies.
引用
收藏
页数:10
相关论文
共 36 条
  • [1] ABRAMAVICIUS D, IN PRESS
  • [2] Energy transfer between semiconductor nanocrystals: Validity of Forster's theory
    Allan, G.
    Delerue, C.
    [J]. PHYSICAL REVIEW B, 2007, 75 (19):
  • [3] Theory of resonance energy transfer involving nanocrystals: The role of high multipoles
    Baer, Roi
    Rabani, Eran
    [J]. JOURNAL OF CHEMICAL PHYSICS, 2008, 128 (18)
  • [4] Coupling and entangling of quantum states in quantum dot molecules
    Bayer, M
    Hawrylak, P
    Hinzer, K
    Fafard, S
    Korkusinski, M
    Wasilewski, ZR
    Stern, O
    Forchel, A
    [J]. SCIENCE, 2001, 291 (5503) : 451 - 453
  • [5] Broken symmetry and quantum entanglement of an exciton in InxGa1-xAs/GaAs quantum dot molecules -: art. no. 075325
    Bester, G
    Zunger, A
    Shumway, J
    [J]. PHYSICAL REVIEW B, 2005, 71 (07):
  • [6] Theory of excitonic spectra and entanglement engineering in dot molecules
    Bester, G
    Shumway, J
    Zunger, A
    [J]. PHYSICAL REVIEW LETTERS, 2004, 93 (04) : 047401 - 1
  • [7] Semiconductor nanocrystals as fluorescent biological labels
    Bruchez, M
    Moronne, M
    Gin, P
    Weiss, S
    Alivisatos, AP
    [J]. SCIENCE, 1998, 281 (5385) : 2013 - 2016
  • [8] Multidimensional femtosecond spectroscopies of molecular aggregates and semiconductor nanostructures: The nonlinear exciton equations
    Chernyak, V
    Zhang, WM
    Mukamel, S
    [J]. JOURNAL OF CHEMICAL PHYSICS, 1998, 109 (21) : 9587 - 9601
  • [9] Third-order optical response of intermediate excitons with fractional nonlinear statistics
    Chernyak, V
    Mukamel, S
    [J]. JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 1996, 13 (06) : 1302 - 1307
  • [10] Interacting excitons described by an infinite series of composite-exciton operators
    Combescot, M.
    Betbeder-Matibet, O.
    [J]. PHYSICAL REVIEW B, 2008, 78 (12)