Observational constraints on recent increases in the atmospheric CH4 burden

被引:421
作者
Dlugokencky, E. J. [1 ]
Bruhwiler, L. [1 ]
White, J. W. C. [2 ]
Emmons, L. K. [3 ]
Novelli, P. C. [1 ]
Montzka, S. A. [1 ]
Masarie, K. A. [1 ]
Lang, P. M. [1 ]
Crotwell, A. M. [1 ,4 ]
Miller, J. B. [1 ,4 ]
Gatti, L. V. [5 ]
机构
[1] NOAA, Earth Syst Res Lab, Boulder, CO 80305 USA
[2] Univ Colorado, Inst Arctic & Alpine Res, Boulder, CO 80309 USA
[3] Natl Ctr Atmospher Res, Div Atmospher Chem, Boulder, CO 80307 USA
[4] Univ Colorado, CIRES, Boulder, CO 80309 USA
[5] IPEN CNEN SP, Div Quim Ambiental, Lab Quim Atmosfer, BR-05508900 Sao Paulo, Brazil
关键词
BIOMASS-BURNING EMISSIONS; METHANE; HYDROXYL;
D O I
10.1029/2009GL039780
中图分类号
P [天文学、地球科学];
学科分类号
07 ;
摘要
Measurements of atmospheric CH4 from air samples collected weekly at 46 remote surface sites show that, after a decade of near-zero growth, globally averaged atmospheric methane increased during 2007 and 2008. During 2007, CH4 increased by 8.3 +/- 0.6 ppb. CH4 mole fractions averaged over polar northern latitudes and the Southern Hemisphere increased more than other zonally averaged regions. In 2008, globally averaged CH4 increased by 4.4 +/- 0.6 ppb; the largest increase was in the tropics, while polar northern latitudes did not increase. Satellite and in situ CO observations suggest only a minor contribution to increased CH4 from biomass burning. The most likely drivers of the CH4 anomalies observed during 2007 and 2008 are anomalously high temperatures in the Arctic and greater than average precipitation in the tropics. Near-zero CH4 growth in the Arctic during 2008 suggests we have not yet activated strong climate feedbacks from permafrost and CH4 hydrates. Citation: Dlugokencky, E.J., et al. (2009), Observational constraints on recent increases in the atmospheric CH4 burden, Geophys. Res. Lett., 36, L18803, doi: 10.1029/2009GL039780.
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页数:5
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