Evaluation of streamwater composition changes in the Vosges Mountains (NE France): 1955-2005

被引:8
作者
Angeli, N. [1 ,2 ]
Dambrine, E. [1 ]
Boudot, J. P. [2 ]
Nedeltcheva, T. [1 ]
Guerold, F. [3 ]
Tixier, G. [3 ]
Probst, A. [4 ]
Party, J. P. [5 ]
Pollier, B. [1 ]
Bourrie, G. [6 ]
机构
[1] INRA, Unite Biogeochim Ecosyst Forestiers, F-54280 Nancy, France
[2] Univ Henry Poincare, Lab Interact Microorganismes Mineraux Mat Organ S, CNRS, Fac Sci,UMR 7137, F-54506 Vandoeuvre Les Nancy, France
[3] Univ Metz, UFR Sci FA, Lab Biodivers & Fonctionnement Ecosyst, F-57070 Metz, France
[4] Univ Toulouse 3, CNRS, UMR 5563, Lab Mecanismes & Transferts Geol, F-31400 Toulouse, France
[5] Sol Conseil, F-67000 Strasbourg, France
[6] INRA, Unite Geochim Sols & Eaux, F-13545 Aix En Provence 04, France
关键词
Stream chemistry; Acidity; Long-term trends; Vosges mountains; SURFACE-WATER CHEMISTRY; NORTH-EASTERN FRANCE; AIR ACT AMENDMENTS; STRENGBACH CATCHMENT; NORTHEASTERN FRANCE; NITROGEN DEPOSITION; SULFATE DEPOSITION; ACIDIC DEPOSITION; TERM CHANGES; LONG-TERM;
D O I
10.1016/j.scitotenv.2009.02.008
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In 1995, in the southwestern Vosges Mountains (NE France), 158 of 395 streams (40%) had a pH lower than 5.5 at baseflow. As elsewhere in Europe, acid deposition has decreased since the seventies, as has base cation deposition. In order to assess the response of streamwater to decreasing deposition, we compared their present chemical composition to their former composition. All comparisons showed a decrease in sulphate concentration. which was greater on granite than on sandstone. In addition calcium, magnesium and aluminium concentrations generally decreased. Acidity in streams draining granite decreased in spring, especially during the eighties, decreases were not observed on sandstone. Continuous monitoring of 5 streams since 1998 confirmed that Al concentrations decreased while changes in pH were small. Chemical trends in streams from the Vosges massif fell between those measured in Northern Europe and Central Europe. This study provides the first broad-scale overview of surface water acidification and recovery in France and emphasizes the need for continuous monitoring to assess long-term changes in aquatic ecosystems. (C) 2009 Elsevier B.V. All rights reserved.
引用
收藏
页码:4378 / 4386
页数:9
相关论文
共 60 条
[1]  
ANGELI N, 2006, THESIS U H POINCARE
[2]  
[Anonymous], 2003, WATER AIR SOIL POLLU
[3]  
Barrett K., 2000, TRANSBOUNDARY ACIDIF, P41
[4]   Evolution of the mineral fertility of an acidic soil during a period of ten years in the Vosges mountains (France). Impact of humus mineralisation [J].
Bonneau, M .
ANNALS OF FOREST SCIENCE, 2005, 62 (03) :253-260
[5]   History of sulfate aerosol radiative forcings [J].
Boucher, O ;
Pham, M .
GEOPHYSICAL RESEARCH LETTERS, 2002, 29 (09) :22-23
[6]  
BOURRIE G, 1978, ACQUISITION COMPOSIT
[7]  
*CITEPA COR, 2005, INV EM POLL ATM FRAN
[8]  
COLIN G, 2003, FORETS FRANCAISES AP, P27
[9]   Evidence of sulphur and nitrogen deposition signals at the United Kingdom Waters Monitoring Network sites [J].
Cooper, DM .
ENVIRONMENTAL POLLUTION, 2005, 137 (01) :41-54
[10]   Evidence of current soil acidification in spruce stands in the Vosges Mountains, north-eastern France [J].
Dambrine, E ;
Pollier, B ;
Poszwa, A ;
Ranger, J ;
Probst, A ;
Viville, D ;
Biron, P ;
Granier, A .
WATER AIR AND SOIL POLLUTION, 1998, 105 (1-2) :43-52