Observation of a Charge Density Wave Incommensuration Near the Superconducting Dome in CuxTiSe2

被引:84
作者
Kogar, A. [1 ,2 ,3 ]
de la Pena, G. A. [1 ,2 ]
Lee, Sangjun [1 ,2 ]
Fang, Y. [2 ]
Sun, S. X. -L. [1 ,2 ]
Lioi, D. B. [4 ]
Karapetrov, G. [4 ]
Finkelstein, K. D. [5 ]
Ruff, J. P. C. [5 ]
Abbamonte, P. [1 ,2 ]
Rosenkranz, S. [3 ]
机构
[1] Univ Illinois, Dept Phys, Urbana, IL 61801 USA
[2] Univ Illinois, Mat Res Lab, Urbana, IL 61801 USA
[3] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA
[4] Drexel Univ, Dept Phys, Philadelphia, PA 19104 USA
[5] Cornell Univ, Cornell High Energy Synchrotron Source, Ithaca, NY 14853 USA
基金
美国国家科学基金会; 美国国家卫生研究院;
关键词
2H-TASE2; 1T-TAS2; PHASE; TISE2;
D O I
10.1103/PhysRevLett.118.027002
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
X-ray diffraction was employed to study the evolution of the charge density wave (CDW) in CuxTiSe2 as a function of copper intercalation in order to clarify the relationship between the CDW and superconductivity. The results show a CDWincommensuration arising at an intercalation value coincident with the onset of superconductivity at around x = 0.055(5). Additionally, it was found that the charge density wave persists to higher intercalant concentrations than previously assumed, demonstrating that the CDW does not terminate inside the superconducting dome. A charge density wave peak was observed in samples up to x = 0.091(6), the highest copper concentration examined in this study. The phase diagram established in this work suggests that charge density wave incommensuration may play a role in the formation of the superconducting state.
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页数:5
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