Light-Driven Ultrafast Polarization Manipulation in a Relaxor Ferroelectric

被引：6

作者：

Park, Suji ^{[1
,3
,4
]}

Wang, Bo ^{[5
]}

Yang, Tiannan ^{[5
]}

Kim, Jieun ^{[6
]}

Saremi, Sahar ^{[6
,7
]}

Zhao, Wenbo ^{[6
]}

Guzelturk, Burak ^{[8
,9
]}

Sood, Aditya

Nyby, Clara

Zajac, Marc

Shen, Xiaozhe ^{[3
]}

Kozina, Michael ^{[3
]}

Reid, Alexander H. ^{[3
]}

Weathersby, Stephen ^{[3
,4
]}

Wang, Xijie ^{[3
]}

Martin, Lane W. ^{[6
,7
]}

Chen, Long-Qing ^{[5
]}

Lindenberg, Aaron M. ^{[1
,2
]}

机构：

[1] Stanford Inst Mat & Energy Sci, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA

[2] Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA

[3] PULSE Inst, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA

[4] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA

[5] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA

[6] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA

[7] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA

[8] Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA

[9] Argonne Natl Lab, Xray Sci Div, 9700 S Cass Ave, Lemont, IL 60439 USA

来源：

NANO LETTERS | 2022年 / 22卷 / 23期

基金：

美国国家科学基金会;

关键词：

ferroelectrics; structural dynamics; ultrafast; electron diffraction; ROTATION;

D O I：

10.1021/acs.nanolett.2c02706

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Relaxor ferroelectrics have been intensely studied for decades based on their unique electromechanical responses which arise from local structural heterogeneity involving polar nanoregions or domains. Here, we report first studies of the ultrafast dynamics and reconfigurability of the polarization in freestanding films of the prototypical relaxor 0.68PbMg1/3Nb2/3O3- 0.32PbTiO3 (PMN-0.32PT) by probing its atomic-scale response via femtosecond-resolution, electron-scattering approaches. By combining these structural measurements with dynamic phase-field simulations, we show that femtosecond light pulses drive a change in both the magnitude and direction of the polarization vector within polar nanodomains on few-picosecond time scales. This study defines new opportunities for dynamic reconfigurable control of the polarization in nanoscale relaxor ferroelectrics.

引用

页码：9275 / 9282

页数：8

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