Excitons in Single-Walled Carbon Nanotubes and Their Dynamics

被引：43
作者：
Amori, Amanda R. [1 ]
Hou, Zhentao [1 ]
Krauss, Todd D. [1 ,2 ]
机构：
[1] Univ Rochester, Dept Chem, Rochester, NY 14627 USA
[2] Univ Rochester, Inst Opt, Rochester, NY 14627 USA
来源：
ANNUAL REVIEW OF PHYSICAL CHEMISTRY, VOL 69 | 2018年 / 69卷
关键词：
single-walled carbon nanotubes; excitons; photoluminescence; ultrafast dynamics; multiple-exciton generation; photon antibunching; DEPENDENT FLUORESCENCE EFFICIENCIES; ABSORPTION CROSS-SECTIONS; SOLAR-CELLS; ELECTRONIC-STRUCTURE; TRANSITION ENERGIES; CARRIER DYNAMICS; WATER-OXIDATION; QUANTUM DOTS; PHOTOLUMINESCENCE; SPECTROSCOPY;
D O I：
10.1146/annurev-physchem-050317-014241
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Understanding exciton dynamics in single-walled carbon nanotubes (SWCNTs) is essential to unlocking the many potential applications of these materials. This review summarizes recent progress in understanding exciton photophysics and, in particular, exciton dynamics in SWCNTs. We outline the basic physical and electronic properties of SWCNTs, as well as bright and dark transitions within the framework of a strongly bound one-dimensional excitonic model. We discuss the many facets of ultrafast carrier dynamics inSWCNTs, including both single-exciton states (bright and dark) and multiple-exciton states. Photophysical properties that directly relate to excitons and their dynamics, including exciton diffusion lengths, chemical and structural defects, environmental effects, and photoluminescence photon statistics as observed through photon antibunching measurements, are also discussed. Finally, we identify a few key areas for advancing further research in the field of SWCNT excitons and photonics.
引用
收藏
页码：81 / 99
页数：19
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