Attosecond photoemission dynamics encoded in real-valued continuum wave functions

被引:15
作者
Gaillac, Romain [1 ,2 ]
Vacher, Morgane [1 ,3 ]
Maquet, Alfred [1 ]
Taieb, Richard [1 ]
Caillat, Jeremie [1 ]
机构
[1] Univ Paris 06, Sorbonne Univ, Lab Chim Phys Mat & Rayonnement, CNRS,UMR 7614, F-75005 Paris, France
[2] Ecole Normale Super, Dept Chem, F-75005 Paris, France
[3] Univ London Imperial Coll Sci Technol & Med, Dept Chem, London SW7 2AZ, England
关键词
DELAY;
D O I
10.1103/PhysRevA.93.013410
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
The dynamics of photoemission is fully encoded in the continuum wave functions selected by the transitions. Using numerical simulations on simple benchmark models, we show how scattering phase shifts and photoemission delays can be retrieved from this unambiguously defined class of wave functions. In contrast with standard scattering waves inherited from collision theory, they are real-valued for one-photon transitions and provide a clear-cut interpretation of the delays recently discussed in the framework of attosecond science.
引用
收藏
页数:6
相关论文
共 41 条
  • [1] Amusia M Y., 1990, Atomic photoeffect
  • [2] [Anonymous], 1999, Quantum Mechanics, Two Volumes Bound as One
  • [3] [Anonymous], 2014, NAT PHOTONICS, V8, P161
  • [4] Bethe H A, 1977, QUANTUM MECH ONE 2 E
  • [5] Attosecond Resolved Electron Release in Two-Color Near-Threshold Photoionization of N2
    Caillat, Jeremie
    Maquet, Alfred
    Haessler, Stefan
    Fabre, Baptiste
    Ruchon, Thierry
    Salieres, Pascal
    Mairesse, Yann
    Taieb, Richard
    [J]. PHYSICAL REVIEW LETTERS, 2011, 106 (09)
  • [6] Multiconfigurational Hartree-Fock close-coupling ansatz: Application to the argon photoionization cross section and delays
    Carette, T.
    Dahlstrom, J. M.
    Argenti, L.
    Lindroth, E.
    [J]. PHYSICAL REVIEW A, 2013, 87 (02):
  • [7] Attosecond spectroscopy in condensed matter
    Cavalieri, A. L.
    Mueller, N.
    Uphues, Th.
    Yakovlev, V. S.
    Baltuska, A.
    Horvath, B.
    Schmidt, B.
    Bluemel, L.
    Holzwarth, R.
    Hendel, S.
    Drescher, M.
    Kleineberg, U.
    Echenique, P. M.
    Kienberger, R.
    Krausz, F.
    Heinzmann, U.
    [J]. NATURE, 2007, 449 (7165) : 1029 - 1032
  • [8] Asymmetry of Wigner's time delay in a small molecule
    Chacon, Alexis
    Lein, Manfred
    Ruiz, Camilo
    [J]. PHYSICAL REVIEW A, 2014, 89 (05):
  • [9] ANGULAR DISTRIBUTION OF PHOTOELECTRONS
    COOPER, J
    ZARE, RN
    [J]. JOURNAL OF CHEMICAL PHYSICS, 1968, 48 (02) : 942 - &
  • [10] Study of attosecond delays using perturbation diagrams and exterior complex scaling
    Dahlstrom, J. M.
    Lindroth, E.
    [J]. JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 2014, 47 (12)