共 47 条
Thermoluminescence of nitrogen-neon and nitrogen-argon nanoclusters immersed in superfluid helium
被引:2
作者:
Meraki, Adil
[1
,2
]
McColgan, Patrick T.
[3
,4
]
Sheludiakov, S.
[3
,4
]
Lee, David M.
[3
,4
]
Khmelenko, Vladimir V.
[3
,4
]
机构:
[1] Bilecik Seyh Edebali Univ, Dept Phys, Bilecik, Turkey
[2] TUBITAK Natl Metrol Inst, Gebze, Turkey
[3] Texas A&M Univ, Dept Phys & Astron, College Stn, TX 77843 USA
[4] Texas A&M Univ, Inst Quantum Sci & Engn, College Stn, TX 77843 USA
关键词:
thermoluminescence;
porous structures;
nanoclusters;
superfluid helium;
ELECTRON-SPIN-RESONANCE;
FROZEN PRODUCTS;
SOLID NITROGEN;
ATOMS;
LUMINESCENCE;
VISUALIZATION;
CONDENSATION;
RELAXATION;
DYNAMICS;
SPECTRA;
D O I:
10.1063/1.5111301
中图分类号:
O59 [应用物理学];
学科分类号:
摘要:
Ensembles of nanoclusters created by injection of nitrogen atoms and molecules as well as rare gas (RG) atoms (Ne and Ar) into superfluid He-4 have been studied via optical and electron spin resonance (ESR) spectroscopies. We studied the dynamics of thermoluminescence spectra emitted during the warming of porous structures formed by nitrogen-neon and nitrogen-argon nanoclusters inside superfluid helium. We show experimental evidence that quantum vortices initiate chemical reactions in porous ensembles of nanoclusters. Using this experimental approach, it is possible to study chemical reactions of heavy atoms and molecules at very low temperatures where normally their diffusion and quantum tunneling in solid matrices are completely suppressed.
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页码:737 / 747
页数:11
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