Nitrogen-Doped Aligned Carbon Nanotube/Graphene Sandwiches: Facile Catalytic Growth on Bifunctional Natural Catalysts and Their Applications as Scaffolds for High-Rate Lithium-Sulfur Batteries

被引:549
作者
Tang, Cheng [1 ]
Zhang, Qiang [1 ]
Zhao, Meng-Qiang [1 ]
Huang, Jia-Qi [1 ]
Cheng, Xin-Bing [1 ]
Tian, Gui-Li [1 ]
Peng, Hong-Jie [1 ]
Wei, Fei [1 ]
机构
[1] Tsinghua Univ, Beijing Key Lab Green Chem React Engn & Technol, Dept Chem Engn, Beijing 100084, Peoples R China
关键词
LI-S BATTERIES; CHEMICAL-VAPOR-DEPOSITION; OXYGEN REDUCTION REACTION; GRAPHENE OXIDE FOAMS; NANOTUBE HYBRIDS; ION BATTERIES; PERFORMANCE; SUPERCAPACITORS; STORAGE; COMPOSITES;
D O I
10.1002/adma.201401243
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Nitrogen-doped aligned CNT/graphene sandwiches are rationally designed and in-situ fabricated by a facile catalytic growth on bifunctional natural catalysts that exhibit high-rate performances as scaffolds for lithium-sulfur batteries, with a high initial capacity of 1152 mA h g(-1) at 1.0 C. A remarkable capacity of 770 mA h g(-1) can be achieved at 5.0 C. Such a design strategy for materials opens up new perspectives to novel advanced functional composites, especially interface-modified hierarchical nanocarbons for broad applications.
引用
收藏
页码:6100 / +
页数:7
相关论文
共 61 条
[51]   The Road for Nanomaterials Industry: A Review of Carbon Nanotube Production, Post-Treatment, and Bulk Applications for Composites and Energy Storage [J].
Zhang, Qiang ;
Huang, Jia-Qi ;
Qian, Wei-Zhong ;
Zhang, Ying-Ying ;
Wei, Fei .
SMALL, 2013, 9 (08) :1237-1265
[52]   Vertically aligned carbon nanotube arrays grown on a lamellar catalyst by fluidized bed catalytic chemical vapor deposition [J].
Zhang, Qiang ;
Zhao, Meng-Qiang ;
Huang, Jia-Qi ;
Liu, Yi ;
Wang, Yao ;
Qian, Wei-Zhong ;
Wei, Fei .
CARBON, 2009, 47 (11) :2600-2610
[53]   Energy-Absorbing Hybrid Composites Based on Alternate Carbon-Nanotube and Inorganic Layers [J].
Zhang, Qiang ;
Zhao, Mengqiang ;
Liu, Yi ;
Cao, Anyuan ;
Qian, Weizhong ;
Lu, Yunfeng ;
Wei, Fei .
ADVANCED MATERIALS, 2009, 21 (28) :2876-+
[54]   Composite Cathodes Containing SWCNT@S Coaxial Nanocables: Facile Synthesis, Surface Modification, and Enhanced Performance for Li-Ion Storage [J].
Zhang, Shu-Mao ;
Zhang, Qiang ;
Huang, Jia-Qi ;
Liu, Xiao-Fei ;
Zhu, Wancheng ;
Zhao, Meng-Qiang ;
Qian, Wei-Zhong ;
Wei, Fei .
PARTICLE & PARTICLE SYSTEMS CHARACTERIZATION, 2013, 30 (02) :158-165
[55]   Unstacked double-layer templated graphene for high-rate lithium-sulphur batteries [J].
Zhao, Meng-Qiang ;
Zhang, Qiang ;
Huang, Jia-Qi ;
Tian, Gui-Li ;
Nie, Jing-Qi ;
Peng, Hong-Jie ;
Wei, Fei .
NATURE COMMUNICATIONS, 2014, 5
[56]   Towards high purity graphene/single-walled carbon nanotube hybrids with improved electrochemical capacitive performance [J].
Zhao, Meng-Qiang ;
Zhang, Qiang ;
Huang, Jia-Qi ;
Tian, Gui-Li ;
Chen, Tian-Chi ;
Qian, Wei-Zhong ;
Wei, Fei .
CARBON, 2013, 54 :403-411
[57]   Graphene/Single-Walled Carbon Nanotube Hybrids: One-Step Catalytic Growth and Applications for High-Rate Li-S Batteries [J].
Zhao, Meng-Qiang ;
Liu, Xiao-Fei ;
Zhang, Qiang ;
Tian, Gui-Li ;
Huang, Jia-Qi ;
Zhu, Wancheng ;
Wei, Fei .
ACS NANO, 2012, 6 (12) :10759-10769
[58]   Hierarchical Nanocomposites Derived from Nanocarbons and Layered Double Hydroxides - Properties, Synthesis, and Applications [J].
Zhao, Meng-Qiang ;
Zhang, Qiang ;
Huang, Jia-Qi ;
Wei, Fei .
ADVANCED FUNCTIONAL MATERIALS, 2012, 22 (04) :675-694
[59]   Highly transparent and conducting ultralarge graphene oxide/single-walled carbon nanotube hybrid films produced by Langmuir-Blodgett assembly [J].
Zheng, Qingbin ;
Zhang, Biao ;
Lin, Xiuyi ;
Shen, Xi ;
Yousefi, Nariman ;
Huang, Zhen-Dong ;
Li, Zhigang ;
Kim, Jang-Kyo .
JOURNAL OF MATERIALS CHEMISTRY, 2012, 22 (48) :25072-25082
[60]   A Graphene-Pure-Sulfur Sandwich Structure for Ultrafast, Long-Life Lithium-Sulfur Batteries [J].
Zhou, Guangmin ;
Pei, Songfeng ;
Li, Lu ;
Wang, Da-Wei ;
Wang, Shaogang ;
Huang, Kun ;
Yin, Li-Chang ;
Li, Feng ;
Cheng, Hui-Ming .
ADVANCED MATERIALS, 2014, 26 (04) :625-631