Enhanced photocatalytic performance of graphene-ZnO nanoplatelet composite thin films prepared by electrostatic spray deposition

被引:64
作者
Joshi, Bhavana N. [1 ]
Yoon, Hyun [1 ]
Na, Seung-Heon [1 ]
Choi, Jae-Young [1 ]
Yoon, Sam S. [1 ]
机构
[1] Korea Univ Anamdong, Sch Mech Engn, Seoul 136713, South Korea
关键词
ZnO; Graphene-ZnO; Photocatalyst; Methylene Blue; SOL-GEL METHOD; ZINC-OXIDE; METHYLENE-BLUE; DEGRADATION; NANOCOMPOSITES; TRANSPARENT; DYES;
D O I
10.1016/j.ceramint.2013.09.060
中图分类号
TQ174 [陶瓷工业]; TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Graphene-ZnO (G-ZnO) composite thin films were produced using the electrostatic spray deposition technique (ESD). The effects of the concentration of graphene and annealing temperature on the structural and photocatalytic properties of the G-ZnO films were studied by X-ray diffraction, scanning electron microscopy, atomic force microscopy, Raman spectroscopy, and UV-visible spectroscopy. We demonstrated that the G-ZnO films exhibit enhanced activities towards the photodegradation of methylene blue dye. A G-ZnO film with 0.1 wt% graphene that was annealed at 300 degrees C showed the highest photo-degradation activity. We found that the incorporation of graphene reduced electron-hole recombination in the ZnO film (C) 2013 Elsevier Ltd and Techna Group S.r.l. All rights reserved.
引用
收藏
页码:3647 / 3654
页数:8
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