Novel hydrophobic PVDF/APTES-GO nanocomposite for natural gas pipelines coating

被引:36
作者
Chiong, S. J. [1 ,2 ]
Goh, P. S. [1 ,2 ]
Ismail, A. F. [1 ,2 ]
机构
[1] Univ Teknol Malaysia, Adv Membrane Technol Res Ctr AMTEC, Skudai 81310, Johor, Malaysia
[2] Univ Teknol Malaysia, FCEE, Johor Baharu 81310, Malaysia
关键词
Polyvinylidene fluoride; 3-Aminopropyltriethoxysilane-graphene oxide; Hydrophobic; Anti-corrosion coating; Natural gas pipelines; GRAPHENE OXIDE; MECHANICAL-PROPERTIES; CORROSION-RESISTANCE; CARBON NANOTUBES; PROTECTIVE-COATINGS; PERFORMANCE; FUNCTIONALIZATION; NANOMATERIAL; FLUORIDE); GRAPHITE;
D O I
10.1016/j.jngse.2017.02.042
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
Polyvinylidene fluoride (PVDF) nanocomposites were successfully prepared by solvent casting approach using graphene oxide (GO) and 3-aminopropyltriethoxysilane-graphene oxide (APTES-GO) as nanofillers. Field emission scanning electron microscope (FESEM) revealed that the PVDF nanocomposites exhibited features of symmetric membrane. Incorporation of 0.4 wt% of APTES-GO into the PVDF matrix led to a significant decrease in wettability with water contact angle (CA) of 102 degrees as compared to 62 for 0.4 wt% GO and 80 for neat PVDF. PVDF/AVIES-GO has increased 2350% in tensile modulus as compared to 75% increased in PVDF/GO nanocomposite. Carbon steel plate, which has similar properties with commercial carbon steel pipelines was used in the salt spray and acid immersion tests. PVDF/APTES-GO nano composite coating was found to exhibit excellent corrosion protection and good adhesion property than other coatings in corrosive environments. (C) 2017 Elsevier B.V. All rights reserved.
引用
收藏
页码:190 / 202
页数:13
相关论文
共 68 条
[1]   Synthesis of Silica Nanoparticles by Sol-Gel: Size-Dependent Properties, Surface Modification, and Applications in Silica-Polymer Nanocomposites-A Review [J].
Ab Rahman, Ismail ;
Padavettan, Vejayakumaran .
JOURNAL OF NANOMATERIALS, 2012, 2012
[2]   Separation Performance of Graphene Oxide Membrane in Aqueous Solution [J].
An, Di ;
Yang, Ling ;
Wang, Ting-Jie ;
Liu, Boyang .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2016, 55 (17) :4803-4810
[3]   Multifunctional Superhydrophobic Polymer/Carbon Nanocomposites: Graphene, Carbon Nanotubes, or Carbon Black? [J].
Asthana, Ashish ;
Maitra, Tanmoy ;
Buechel, Robert ;
Tiwari, Manish K. ;
Poulikakos, Dimos .
ACS APPLIED MATERIALS & INTERFACES, 2014, 6 (11) :8859-8867
[4]   FP-based formulations as protective coatings in oil/gas pipelines [J].
Bayram, Tamer Can ;
Orbey, Nese ;
Adhikari, Ramesh Y. ;
Tuominen, Mark .
PROGRESS IN ORGANIC COATINGS, 2015, 88 :54-63
[5]  
Branch Mahshahr., 2012, International Journal of Innovation and Applied Studies, V1, P186
[6]   Novel anticorrosion coatings prepared from polyaniline/graphene composites [J].
Chang, Chi-Hao ;
Huang, Tsao-Cheng ;
Peng, Chih-Wei ;
Yeh, Tzu-Chun ;
Lu, Hsin-I ;
Hung, Wei-I ;
Weng, Chang-Jian ;
Yang, Ta-I ;
Yeh, Jui-Ming .
CARBON, 2012, 50 (14) :5044-5051
[7]   Advanced anticorrosive coatings prepared from electroactive polyimide/graphene nanocomposites with synergistic effects of redox catalytic capability and gas barrier properties [J].
Chang, K. C. ;
Hsu, C. H. ;
Lu, H. I. ;
Ji, W. F. ;
Chang, C. H. ;
Li, W. Y. ;
Chuang, T. L. ;
Yeh, J. M. ;
Liu, W. R. ;
Tsai, M. H. .
EXPRESS POLYMER LETTERS, 2014, 8 (04) :243-255
[8]   Graphene Oxide: Preparation, Functionalization, and Electrochemical Applications [J].
Chen, Da ;
Feng, Hongbin ;
Li, Jinghong .
CHEMICAL REVIEWS, 2012, 112 (11) :6027-6053
[9]   An improved Hummers method for eco-friendly synthesis of graphene oxide [J].
Chen, Ji ;
Yao, Bowen ;
Li, Chun ;
Shi, Gaoquan .
CARBON, 2013, 64 :225-229
[10]   A design of gradient interphase reinforced by silanized graphene oxide and its effect on carbon fiber/epoxy interface [J].
Chen, Lei ;
Jin, Hao ;
Xu, Zhiwei ;
Shan, Mingjing ;
Tian, Xu ;
Yang, Caiyun ;
Wang, Zhen ;
Cheng, Bowen .
MATERIALS CHEMISTRY AND PHYSICS, 2014, 145 (1-2) :186-196